Dynamics of Polar Vortex Crystallization.

Phys Rev Lett

Smart Ferroic Materials Center, Physics Department and Institute for Nanoscience and Engineering, University of Arkansas, Fayetteville, Arkansas 72701, USA.

Published: August 2024

Vortex crystals are commonly observed in ultrathin ferroelectrics. However, a clear physical picture of origin of this topological state is currently lacking. Here, we show that vortex crystallization in ultrathin Pb(Zr_{0.4},Ti_{0.6})O_{3} films stems from the softening of a phonon mode and can be described as a Z_{2}×SU(1) symmetry-breaking transition. This result sheds light on the topology of the polar vortex patterns and bridges polar vortices with smectic phases, spin spirals, and other modulated states. Finally, we predict a resonant switching of the vortex tube orientation driven by midinfrared laser light which could enable new technologies.

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http://dx.doi.org/10.1103/PhysRevLett.133.096801DOI Listing

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