AI Article Synopsis
- The latest advancement in perovskite solar cell (PSC) technology focuses on a new technique called thermal imprinting-assisted ion exchange passivation (TIAIEP) that targets surface defects.
- TIAIEP enhances the performance of PSCs by using a passivator to promote ion exchange specifically at defect sites, creating a compositional gradient that minimizes charge recombination.
- Devices treated with TIAIEP achieve a power conversion efficiency of 22.29% and display impressive longevity, retaining 91% efficiency after 2000 hours of storage and 90% after 1200 hours of continuous light exposure.
Article Abstract
The latest development in perovskite solar cell (PSC) technology has been significantly influenced by advanced techniques aimed at passivating surface defects. This work presents a new approach called thermal imprinting-assisted ion exchange passivation (TIAIEP), which delivers a different approach to conventional solution-based methods. TIAIEP focuses on addressing surface imperfections in solid-state films by using a passivator that promotes ion exchange specifically at the defect sites within the perovskite layer. By adjusting the time and temperature of the TIAIEP process, we achieve substantial enhancement in the creation of a compositional gradient within the films. This optimization slows the cooling rate of hot carriers, leading to minimizing charge recombination and improving the device performance. Remarkably, devices treated with TIAIEP achieve a 22.29% power conversion efficiency and show outstanding stability, with unencapsulated PSCs maintaining 91% of their original efficiency after over 2000 h of storage and 90% efficiency after 1200 h of constant illumination. These results highlight TIAIEP's effectiveness in mitigating surface defects, improving both the photoelectric and stability performance of PSCs, and indicating significant potential for large-scale application in perovskite film passivation, promoting the widespread adoption of this technology.
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| http://dx.doi.org/10.1021/acsami.4c08538 | DOI Listing |
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