Driven Self-Assembly of Patchy Particles Overcoming Equilibrium Limitations.

J Chem Theory Comput

Department of Biomedical Engineering, Faculty of Engineering, Tel Aviv University, Tel Aviv 6997801, Israel.

Published: September 2024

Bridging biological complexity and synthetic material design, we investigate dissipative self-assembly in patchy particle systems. Utilizing Monte Carlo and Molecular Dynamics simulations, we demonstrate how external driving forces mitigate equilibrium trade-offs between assembly time and structural stability, traditionally encountered in self-assembly processes. Our findings also extend to biological-mimicking environments, where we explore the dynamics of patchy particles under crowded conditions. This comprehensive analysis offers insights into advanced material design, opening avenues for innovations in nanotechnology applications.

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Source
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC11428128PMC
http://dx.doi.org/10.1021/acs.jctc.4c01118DOI Listing

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