Liquid phase direct amination of phenols to primary anilines with hydrazine was achieved using commercial NiLa-perovskite catalysts as bifunctional Lewis acid/redox-active catalysts without adding any external hydride sources. The amination strategy took place efficiently in the absence of any amount of reducing gasses (H/NH) and noble metals under mild conditions.
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Nickel-based perovskite-catalysed direct phenol-to-aniline liquid-phase transformations.
Chem Commun (Camb)
September 2024
Department of Applied and Environmental Chemistry and Interdisciplinary Excellence Centre, Institute of Chemistry, University of Szeged, Rerrich Béla tér 1, Szeged, H-6720, Hungary.
Liquid phase direct amination of phenols to primary anilines with hydrazine was achieved using commercial NiLa-perovskite catalysts as bifunctional Lewis acid/redox-active catalysts without adding any external hydride sources. The amination strategy took place efficiently in the absence of any amount of reducing gasses (H/NH) and noble metals under mild conditions.
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