The oscillatory retinal neuron (ORN) is a promising technology for achieving in-sensor cognitive image computing without external power. While its operation is based on photoinduced negative differential resistance (NDR) at a graphene/silicon interface to directly convert the incident optical signal into voltage oscillations, the optoelectronic mechanism of the NDR remains elusive. Here, nonadiabatic quantum molecular dynamics simulations show that the interplay of band alignment and charge transfer rates of photoexcited carriers at varying applied voltages gives rise to NDR at a graphene/silicon interface under illumination. Such intrinsic NDR at an interface, along with extrinsic circuit-level factors, could enable the much needed rational design of desired image computing functionality of ORN devices in the era of ubiquitous AI on edge devices.
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http://dx.doi.org/10.1021/acs.jpclett.4c02272 | DOI Listing |
J Phys Chem Lett
September 2024
Collaboratory for Advanced Computing and Simulation, University of Southern California, Los Angeles, California 90089-0242, United States.
Materials (Basel)
April 2024
Consiglio Nazionale delle Ricerche, Istituto per la Microelettronica e i Microsistemi, Via P. Gobetti 101, 40129 Bologna, Italy.
Graphene-silicon Schottky diodes are intriguing devices that straddle the border between classical models and two-dimensional ones. Many papers have been published in recent years studying their operation based on the classical model developed for metal-silicon Schottky diodes. However, the results obtained for diode parameters vary widely in some cases showing very large deviations with respect to the expected range.
View Article and Find Full Text PDFMaterials (Basel)
March 2024
Institute of Laser Engineering, Osaka University, Osaka 565-0871, Japan.
Graphene shows great potential in developing the next generation of electronic devices. However, the real implementation of graphene-based electronic devices needs to be compatible with existing silicon-based nanofabrication processes. Characterizing the properties of the graphene/silicon interface rapidly and non-invasively is crucial for this endeavor.
View Article and Find Full Text PDFNanomaterials (Basel)
February 2024
School of Materials Science and Engineering, Chang'an University, Xi'an 710061, China.
Graphene/silicon heterojunction photodetectors suffer from a high dark current due to the high surface states and low barrier height at the interface, which limits their application. In this study, we introduce an HfO interfacial layer via magnetron sputtering to address this issue. With this new structure, the dark current is reduced by six times under a bias voltage of -2 V.
View Article and Find Full Text PDFNanomaterials (Basel)
May 2023
School of Electronic Science and Engineering, Xiamen University, Xiamen 361102, China.
Graphene/silicon (Si) heterojunction photodetectors are widely studied in detecting of optical signals from near-infrared to visible light. However, the performance of graphene/Si photodetectors is limited by defects created in the growth process and surface recombination at the interface. Herein, a remote plasma-enhanced chemical vapor deposition is introduced to directly grow graphene nanowalls (GNWs) at a low power of 300 W, which can effectively improve the growth rate and reduce defects.
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