A one-step synthesis of porphyrin-silver acetylide clusters from tetra alkyne-substituted porphyrin is described. The solid-state properties of three 2D-like compounds were fully characterised using XPS and XRD while their catalytic properties under CO electroreduction reaction conditions were assessed and their faradaic efficiency quantified.
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Porphyrin-silver acetylide cluster catalysts with dual active sites for the electrochemical reduction of CO.
Chem Commun (Camb)
September 2024
Universite de Pau et Pays de l'Adour, E2S UPPA, CNRS, IPREM UMR 5254 Technopole Hélioparc 2 avenue du Président Pierre Angot, 64053 PAU CEDEX 09, France.
A one-step synthesis of porphyrin-silver acetylide clusters from tetra alkyne-substituted porphyrin is described. The solid-state properties of three 2D-like compounds were fully characterised using XPS and XRD while their catalytic properties under CO electroreduction reaction conditions were assessed and their faradaic efficiency quantified.
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