Exposure to polycyclic aromatic hydrocarbons (PAHs) in the Chinese population was among the highest globally and associated with various adverse effects. This study examines the impact of China's two-phase clean air initiatives, namely the Air Pollution Prevention and Control Action Plan (APPCAP) in 2013-2017 and the Blue-Sky Defense War (BSDW) in 2018-2020, on PAH levels and human exposures in Beijing. To evaluate the effects of APPCAP, we measured 16 PAHs in 287 PM samples collected in Beijing and 9 PAH metabolites in 358 urine samples obtained from 54 individuals who traveled from Los Angeles to Beijing between 2014 and 2018. The concentration of PM-bound benzo[a]pyrene equivalents (BaPeq) decreased by 88.5% in 2014-2018 due to reduced traffic, coal, and biomass emissions. PAH metabolite concentrations in travelers' urine decreased by 52.3% in Beijing, correlated with changes in PM and NO levels. In contrast, no significant changes were observed in Los Angeles. To evaluate BSDW's effects, we collected 123 additional PM samples for PAH measurements in 2019-2021. We observed sustained reductions in BaPeq concentrations attributable to reductions in coal and biomass emissions during the BSDW phase, but those from traffic sources remained unchanged. After accounting for meteorological factors, China's two-phase clean air initiatives jointly reduced Beijing's PM-bound BaPeq concentrations by 96.6% from 2014 to 2021. These findings provide compelling evidence for the effectiveness of China's clean air actions in mitigating population exposure to PAHs in Beijing.
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http://dx.doi.org/10.1016/j.scib.2024.08.015 | DOI Listing |
Adv Mater
December 2024
Key Laboratory of Applied Surface and Colloid Chemistry, Ministry of Education, Shaanxi Key Laboratory for Advanced Energy Devices, Shaanxi Engineering Lab for Advanced Energy Technology School of Materials Science and Engineering, Shaanxi Normal University, Xi'an, 710119, P. R. China.
The rapidly increased efficiency of perovskite solar cells (PSCs) indicates their broad commercial prospects, but the commercialization of perovskite faces complex optimization processes and stability issues. In this work, a simple optimized strategy is developed by the addition of trimethylgermanium chloride (TGC) into FACsPbI precursor solution. TGC triggers the successive interactions in perovskite solution and film, involving the hydrolysis of vulnerable Ge─Cl bond forming Ge─OH group, then forming the hydrogen bonds (O─H···N and O─H···I) with FAI.
View Article and Find Full Text PDFWater Res
December 2024
Faculty of Applied Science, School of Engineering, University of British Columbia Okanagan Campus, Kelowna, British Columbia V1V 1V7, Canada.
In this research, a sustainable blue-green infrastructure (BGI) was developed to efficiently remove contaminants from stormwater through a combined use of modified porous asphalt (PA) and microalgae cultivation to provide a potential drinking water (DW) source. According to the results, the modified PA with powder activated carbon (PAC) could successfully reduce the level of total suspended solids (TSS), turbidity, polycyclic aromatic hydrocarbons (PAHs), oil and grease to below the DW standards but failed to efficiently remove some heavy metals (HMs) and nutrient pollutants. The results revealed that the treated stormwater was an appropriate medium for microalgae cultivation.
View Article and Find Full Text PDFLancet Reg Health West Pac
December 2024
School of Biomedical Convergence Engineering, College of Information and Biomedical Engineering, Pusan National University, Yangsan, South Korea.
Background: Little is known about the impact of PM on people with disabilities. We aimed to explore the association between PM and hospitalization via the emergency department (ED admission) among people with disabilities, together with the attributable ED admission cases and costs.
Methods: We applied a time-stratified case-crossover design adjusting ozone, holiday, and temperature using seven years (2015-2021) of claim-based data on ED admissions from the Korean National Health Insurance Database.
Anal Chem
December 2024
School of Chemistry, University of Bristol, Bristol BS8 1TS, United Kingdom.
Aerosol droplets are unique microcompartments containing microscopic amounts of material and exhibiting surprising chemical reactivity. Although a diverse set of tools exists to characterize the chemical composition of individual submicron particles in air, comparatively fewer approaches can chemically analyze individual, airborne picolitre droplets. We describe a novel approach for mass spectrometric analysis of individual aqueous picolitre droplets (∼2-180 pL volume) containing down to ∼1 pg analyte mass per droplet.
View Article and Find Full Text PDFJ Environ Manage
December 2024
Institute of Geographical Sciences and Natural Resources, Chinese Academy of Science, No.11 Datunjia, Chaoyang, Beijing, 100101, PR China. Electronic address:
In the context of emphasizing on the food production, clean air guarding and sustainable development of agriculture, straw returning practices have been widely promoted, however, most studies have not linked straw returning adoption and smallholder's agricultural income in double-season rice cropping system. Based on a face-to-face survey data from 797 farmers in Jianghan Plain, Central China, we filled this gap by using the endogenous switching regression model to estimate the impact of farmer's straw returning on their agricultural income. The evidences show number of family laborers and technical training are the main factors influencing farmers' adoption of SR.
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