Functional composite layers composed of an amino-functionalized zirconium 1,4-dicarboxybenzene metal-organic framework were constructed on zinc anodes to mitigate the interface disturbances in aqueous batteries. These layers enable robust Zn adsorption and homogenized Zn transport and deposition kinetics, facilitating achieving high stability in a symmetric cell (3500 h) and a full cell (35 000 cycles, 96.7%).
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