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Coassembly of Complementary Polyhedral Metal-Organic Framework Particles into Binary Ordered Superstructures. | LitMetric

AI Article Synopsis

  • Researchers created a new type of 3D structural arrangement using two different types of metal-organic framework (MOF) particles that fit together well based on their sizes, shapes, and charges.
  • They used a special technique called polymeric-attenuated Coulombic self-assembly, which helped them also combine these MOF particles with spherical polystyrene particles to form 2D structures.
  • The findings open up possibilities for using MOFs to design complex superstructures made from particles of diverse sizes, shapes, and material types.

Article Abstract

Here we report the formation of a 3D NaCl-type binary porous superstructure coassembly of two colloidal polyhedral metal-organic framework (MOF) particles having complementary sizes, shapes, and charges. We employed a polymeric-attenuated Coulombic self-assembly approach, which also facilitated the coassembly of these MOF particles with spherical polystyrene particles to form 2D binary superstructures. Our results pave the way for using MOFs to create sophisticated superstructures comprising particles of various sizes, shapes, porosities, and chemical compositions.

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Source
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC11311218PMC
http://dx.doi.org/10.1021/jacs.4c07194DOI Listing

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