China, the Unite States (US), the European Union (EU), India, and Russia are the world's top 5 fossil fuel and cement CO (FFC) emitting countries or regions (CRs). It is very important to understand their status of carbon neutrality, and to monitor their future changes of net carbon fluxes (NCFs). In this study, we implemented a well-established global carbon assimilation system (GCAS, Version 2) to infer global surface carbon fluxes from May 2009 to December 2019 using both GOSAT and OCO-2 XCO retrievals. The reductions of flux uncertainty and XCO bias, and the evaluation of posterior flux show that GCAS has comparable and good performance in the 5 CRs. The results suggest that Russia has achieved carbon neutrality, but the other 4 are still far from being carbon neutral, especially China. The mean annual NCFs in China, the US, the EU, India, and Russia are 2.33 ± 0.29, 0.82 ± 0.20, 0.42 ± 0.16, 0.50 ± 0.12, and -0.33 ± 0.23 PgC yr, respectively. From 2010 to 2019, the NCFs showed an increasing trend in the US and India, a slight downward trend after 2013 in China, and were stable in the EU. The changes of land sinks in China and the US might be the main reason for their trends. India's trend was mainly due to the increase of FFC emission. The relative contributions of NCFs to the global land net carbon emission of China and the EU have decreased, while those of the US and India have increased, implying the US and India must take more active measures to control carbon emissions or increase their sinks. This study indicates that satellite XCO could be successfully used to monitor the changes of regional NCFs, which is of great significance for major countries to achieve greenhouse gas control goals.
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http://dx.doi.org/10.1016/j.fmre.2022.02.001 | DOI Listing |
Sci Rep
January 2025
State-owned Jiaozuo Forest Farm, Jiaozuo, 454000, Henan, China.
Accurately estimating forest carbon sink and exploring their climate-driven mechanisms are critical to achieving carbon neutrality and sustainable development. Fewer studies have used machine learning-based dynamic models to estimate forest carbon sink. The climate-driven mechanisms in Shangri-La have yet to be explored.
View Article and Find Full Text PDFEnviron Res
January 2025
School of Materials and Chemistry, University of Shanghai for Science and Technology, Shanghai 200093, China. Electronic address:
The pressing necessity to mitigate climate change and decrease greenhouse gas emissions has driven the advancement of heterostructure-based photocatalysts for effective CO₂ reduction. This study introduces a novel heterojunction photocatalyst formed by integrating potassium-doped polymeric carbon nitride (KPCN) with metallic Zn₃N₂, synthesized via a microwave-assisted molten salt method. The resulting Schottky contact effectively suppresses the reverse diffusion of electrons, achieving spatial separation of photogenerated charges and prolonging their lifetime, which significantly enhances photocatalytic activity and efficiency.
View Article and Find Full Text PDFJ Environ Manage
January 2025
School of Petroleum, China University of Petroleum-Beijing at Karamay, Karamay, China.
Carbon neutrality has gained considerable attention globally, and the impact of environmental policy on businesses has been extensively studied. However, the mechanism through which environmental policy affects production efficiency within the enterprise remains unclear. The objectives of this paper are: 1.
View Article and Find Full Text PDFJ Colloid Interface Sci
December 2024
Laboratory of Alternative Energy Conversion Systems, Department of Mechanical Engineering, School of Engineering, University of Thessaly, Pedion Areos 38834, Greece. Electronic address:
The coupling of carbon dioxide (CO) with epoxides to produce cyclic carbonates is a desirable decarbonization approach, but its commercial applicability is still restricted by the costly catalysts required, as well as the need for high temperature and high pressure. Herein, oxygen vacancy-rich defective tungsten oxide (WO) rich in Lewis acid sites was modified by Prussian blue (PB), and the obtained composite reaches up to 94 % styrene carbonate yield (171 mmol gh) at ambient temperature and pressure, exhibiting outstanding advantages in the photocatalytic CO cycloaddition reaction compared with currently reported photocatalysts. It is found that the introduction of PB with photothermal properties significantly enhances the capability of WO to absorb and activate CO and epoxide, along with its light utilization ability.
View Article and Find Full Text PDFSci Adv
January 2025
Department of Cardiac Surgery, Peking University Third Hospital, Beijing 100191, China.
Following myocardial infarction (MI), the accumulation of CD86-positive macrophages in the ischemic injury zone leads to secondary myocardial damage. Precise pharmacological intervention targeting this process remains challenging. This study engineered a nanotherapeutic delivery system with CD86-positive macrophage-specific targeting and ultrasound-responsive release capabilities.
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