Plasmons in the Kagome metal CsVSb.

Nat Commun

Department of Physics, Florida State University, Tallahassee, FL, 32306, USA.

Published: June 2024

AI Article Synopsis

  • Plasmon polaritons are oscillations of electrons interacting with electromagnetic fields, allowing for the creation of new devices that can manipulate light at very small scales, but research is limited in correlated materials like the Kagome metal CsVSb.* -
  • The study utilizes infrared nano-imaging to observe plasmon waves in thin flakes of CsVSb, finding that the wavelength can vary based on the thickness of the flakes.* -
  • Results indicate that electronic correlations may have altered the properties of the surface plasmons, enhancing their stability and leading to a transition into hyperbolic bulk plasmons with reduced energy loss.*

Article Abstract

Plasmon polaritons, or plasmons, are coupled oscillations of electrons and electromagnetic fields that can confine the latter into deeply subwavelength scales, enabling novel polaritonic devices. While plasmons have been extensively studied in normal metals or semimetals, they remain largely unexplored in correlated materials. In this paper, we report infrared (IR) nano-imaging of thin flakes of CsVSb, a prototypical layered Kagome metal. We observe propagating plasmon waves in real-space with wavelengths tunable by the flake thickness. From their frequency-momentum dispersion, we infer the out-of-plane dielectric function that is generally difficult to obtain in conventional far-field optics, and elucidate signatures of electronic correlations when compared to density functional theory (DFT). We propose correlation effects might have switched the real part of from negative to positive values over a wide range of middle-IR frequencies, transforming the surface plasmons into hyperbolic bulk plasmons, and have dramatically suppressed their dissipation.

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Source
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC11199534PMC
http://dx.doi.org/10.1038/s41467-024-49723-xDOI Listing

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