One-dimensional transition metal dichalcogenides exhibiting an enhanced bulk photovoltaic effect have the potential to exceed the Shockley-Queisser limit efficiency in solar energy harvest within - junction architectures. However, the collective output of these prototype devices remains a challenge. We report on the synthesis of single-crystalline WS ribbon arrays with defined chirality and coherent polarity through an atomic manufacturing strategy. The chirality of WS ribbon was defined by substrate couplings into tunable armchair, zigzag, and chiral species, and the polarity direction was determined by the ribbon-precursor interfacial energy along a coherent direction. A single armchair ribbon showed strong bulk photovoltaic effect and the further integration of ~1000 aligned ribbons with coherent polarity enabled upscaling of the photocurrent.
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http://dx.doi.org/10.1126/science.adn9476 | DOI Listing |
Anal Chem
January 2025
Institute for Advanced Optics, Hunan Institute of Science and Technology, Yueyang, Hunan 414006, China.
Diffraction imaging of cells allows rapid phenotyping by the response of intracellular molecules to coherent illumination. However, its ability to distinguish numerous types of human leukocytes remains to be investigated. Here, we show that accurate classification of three lymphocyte subtypes can be achieved with features extracted from cross-polarized diffraction image (p-DI) pairs.
View Article and Find Full Text PDFProc Natl Acad Sci U S A
January 2025
Department of Materials Science and Engineering, Stanford University, Stanford, CA 94305.
A central paradigm of nonequilibrium physics concerns the dynamics of heterogeneity and disorder, impacting processes ranging from the behavior of glasses to the emergent functionality of active matter. Understanding these complex mesoscopic systems requires probing the microscopic trajectories associated with irreversible processes, the role of fluctuations and entropy growth, and the timescales on which nonequilibrium responses are ultimately maintained. Approaches that illuminate these processes in model systems may enable a more general understanding of other heterogeneous nonequilibrium phenomena, and potentially define ultimate speed and energy cost limits for information processing technologies.
View Article and Find Full Text PDFSensors (Basel)
December 2024
Institute of Mechanical Intelligence, Scuola Superiore Sant'Anna, Via G. Moruzzi 1, 56124 Pisa, Italy.
CloudSim is a versatile simulation framework for modeling cloud infrastructure components that supports customizable and extensible application provisioning strategies, allowing for the simulation of cloud services. On the other hand, Distributed Acoustic Sensing (DAS) is a ubiquitous technique used for measuring vibrations over an extended region. Data handling in DAS remains an open issue, as many applications need continuous monitoring of a volume of samples whose storage and processing in real time require high-capacity memory and computing resources.
View Article and Find Full Text PDFMaterials (Basel)
December 2024
Department of Chemistry, Materials and Chemical Engineering "Giulio Natta", Politecnico di Milano, Via Mancinelli 7, 20131 Milan, Italy.
The aim of the present work is to study the atmospheric corrosion behavior of metals exposed to both urban (Milan, IT-Lombardia) and marine (Bonassola, IT-Liguria) atmospheres in Italy. A number of coupons (100 × 150 mm) of carbon steel (CS), hot-dip galvanized steel (GS) and different grades of stainless steel (SS) were exposed. At fixed periods of time, samples were characterized by means of Linear Polarization Resistance (LPR), mass loss tests and corrosion product analysis.
View Article and Find Full Text PDFJ Chem Phys
January 2025
Center for Quantum and Topological Systems, New York University Abu Dhabi, P.O. Box 129188, Abu Dhabi, United Arab Emirates.
Pulsed dynamic nuclear polarization (DNP) enhances the nuclear magnetic resonance sensitivity by coherently transferring electron spin polarization to dipolar coupled nuclear spins. Recently, many new pulsed DNP techniques such as NOVEL, TOP, XiX, TPPM, and BEAM have been introduced. Despite significant progress, numerous challenges remain unsolved.
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