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On-Chip Stimulated Raman Scattering Imaging and Quantification of Molecular Diffusion in Aqueous Microfluidics.
Anal Chem
January 2025
State Key Laboratory of Surface Physics and Department of Physics, Academy for Engineering and Technology, Key Laboratory of Micro and Nano Photonic Structures (Ministry of Education), Shanghai Key Laboratory of Metasurfaces for Light Manipulation, Fudan University, Shanghai 200433, China.
Numerous chemical reactions and most life processes occur in aqueous solutions, where the physical diffusion of small molecules plays a vital role, including solvent water molecules, solute biomolecules, and ions. Conventional methods of measuring diffusion coefficients are often limited by technical complexity, large sample consumption, or significant time cost. Here, we present an optical imaging method to study molecular diffusion by combining stimulated Raman scattering (SRS) microscopy with microfluidics: a "Y"-shaped microfluidic channel forming two laminar flows with a stable concentration gradient across the interface.
View Article and Find Full Text PDFWe present the first, to our knowledge, metasurface holographic display method with exceptional fidelity and minimal edge noise, based on highly uniform flat-top light generated by a digital micromirror device (DMD). Based on the error-diffusion algorithm and iterative refinement process, the amplitude distribution of the initial Gaussian light was dynamically closed-loop modulated, and the standard difference of the intensity of the 3 mm diameter center flat-top beam was reduced to less than 3.4%.
View Article and Find Full Text PDFAchiral metasurfaces with near-field optical chirality have attracted great attention in molecular sensing and chiral emission control. Here, the circular dichroism (CD) response of an achiral metasurface induced by spatially selective coupling with polymethyl methacrylate (PMMA) molecules is demonstrated. A designed achiral metasurface with a V-shaped resonator exhibits large optical chirality with a strongly dissymmetric distribution under circular polarization.
View Article and Find Full Text PDFAdjoint method-based Fourier neural operator surrogate solver for wavefront shaping in tunable metasurfaces.
iScience
January 2025
Department of Artificial Intelligence, Hanyang University, Seoul 04763, South Korea.
We present a Fourier neural operator (FNO)-based surrogate solver for the efficient optimization of wavefronts in tunable metasurface controls. Existing methods, including the Gerchberg-Saxton algorithm and the adjoint optimization, are often computationally demanding due to their iterative processes, which require numerical simulations at each step. Our surrogate solver overcomes this limitation by providing highly accurate gradient estimations with respect to changes in tunable meta-atoms without the need for direct simulations.
View Article and Find Full Text PDFPhotoreconfigurable Metasurface for Independent Full-Space Control of Terahertz Waves.
Sensors (Basel)
December 2024
Research Center of Applied Electromagnetics, Nanjing University of Information Science and Technology, Nanjing 210044, China.
We present a novel photoreconfigurable metasurface designed for independent and efficient control of electromagnetic waves with identical incident polarization and frequency across the entire spatial domain. The proposed metasurface features a three-layer architecture: a top layer incorporating a gold circular split ring resonator (CSRR) filled with perovskite material and dual -shaped perovskite resonators; a middle layer of polyimide dielectric; and a bottom layer comprising a perovskite substrate with an oppositely oriented circular split ring resonator filled with gold. By modulating the intensity of a laser beam, we achieve autonomous manipulation of incident circularly polarized terahertz waves in both transmission and reflection modes.
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