Recent developments have led to the possibility of embedding machine learning tools into experimental platforms to address key problems, including the characterization of the properties of quantum states. Leveraging on this, we implement a quantum extreme learning machine in a photonic platform to achieve resource-efficient and accurate characterization of the polarization state of a photon. The underlying reservoir dynamics through which such input state evolves is implemented using the coined quantum walk of high-dimensional photonic orbital angular momentum and performing projective measurements over a fixed basis. We demonstrate how the reconstruction of an unknown polarization state does not need a careful characterization of the measurement apparatus and is robust to experimental imperfections, thus representing a promising route for resource-economic state characterization.
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http://dx.doi.org/10.1103/PhysRevLett.132.160802 | DOI Listing |
J Phys Chem Lett
January 2025
International Tomography Center, SB RAS, 3A Institutskaya St., Novosibirsk 630090, Russia.
Nuclear magnetic resonance is extremely attractive for operando studies of chemical reactors. However, the heterogeneous catalyst particles placed inside an NMR probe greatly affect the uniformity of the magnetic field. This problem is especially acute when studying heterogeneous hydrogenation processes using parahydrogen.
View Article and Find Full Text PDFR Soc Open Sci
January 2025
Pharmaceutical Analytical Chemistry Department, Faculty of Pharmacy, Cairo University, Cairo 11562, Egypt.
Carbon quantum dots (CQDs) are a recently developed class of fluorescent nanoparticles made from carbon. Co-doping with heteroatoms such as nitrogen and sulfur improved the properties and generated a high quantum yield. In the proposed study, we utilized a simple, cost-effective, single-stage hydrothermal approach to produce extreme photoluminescence co-doped, nitrogen and sulfur, CQDs (N,S-CODs).
View Article and Find Full Text PDFJ Phys Chem A
January 2025
School of Physical Science and Technology, Southwest University, Chongqing 400715, China.
Searching for single-molecule magnets (SMM) with large effective blocking barriers, long relaxation times, and high magnetic blocking temperatures is vitally important not only for the fundamental research of magnetism at the molecular level but also for the realization of new-generation magnetic memory unit. Actinides (An) atoms possess extremely strong spin-orbit coupling (SOC) due to their 5 orbitals, and their ground multiplets are largely split into several sublevels because of the strong interplay between the SOC of An atoms and the crystal field (CF) formed by ligand atoms. Compared to TM-based SMMs, more dispersed energy level widths of An-based SMMs will give a larger total zero field splitting (ZFS) and thus provide a necessary condition to derive a higher .
View Article and Find Full Text PDFLight Sci Appl
January 2025
State Key Laboratory of Advanced Optical Communication Systems and Networks, School of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai, 200240, China.
Non-Hermitian topological photonics plays a key role in bridging topological matter with gain and loss engineering in optics. Here we report the experimental observation of the break of chiral currents in a Hall ladder from the non-Hermiticity by constructing synthetic frequency dimension in two rings, where currents on both legs of the ladder co-propagate in the same direction. The origin of such phenomena is resulted from the interplay between the effective magnetic flux and the on-site gain and loss.
View Article and Find Full Text PDFMaterials (Basel)
December 2024
School of Physics and Electronic-Information Engineering, Hubei Engineering University, Xiaogan 432000, China.
In order to promote power conversion efficiency and reduce energy loss, we propose a perovskite solar cell based on cylindrical MAPbI3 microstructure composed of a MAPbI perovskite layer and a hole transport layer (HTL) composed of PEDOT:PSS. According to the charge transport theory, which effectually increases the contact area of the HTL, promoting the electronic transmission capability, the local field enhancement and scattering effects of the surface plasmon polaritons help to couple the incident light to the solar cell, which can increase the absorption of light in the active layer of the solar cell and improve its light absorption efficiency (LAE). based on simulation results, a cylindrical microstructure of the perovskite layer increases the contact area of the hole transport layer, which could improve light absorption, quantum efficiency (QE), short-circuit current density (J), and electric power compared with the perovskite layer of other structures.
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