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Hypothesis: The formation of soft colloidal crystals, which are nonclose-packed ordered arrays of colloidal particles suspended in a solvent, is dictated by a single physical factor that yields a fixed threshold at order-disorder boundaries for different experimental conditions such as ion concentration, solvent type, and particle size. Identifying the determinant factor and its threshold value should enable the prediction of the critical concentrations of colloidal particles to form soft colloidal crystals.
Experiments: Soft colloidal crystals were fabricated using a series of monohydric alcohols as dispersion media and reflectance spectra were measured to locate order-disorder boundaries. The interaction forces acting between particles were also measured by employing atomic force microscopy.
Findings: The interparticle forces at the order-disorder boundaries exhibited a universal threshold that was independent of the solvent types including alcohols and water. Therefore, the determinant factor for the formation of soft colloidal crystals was determined to be the force acting between the particles. Furthermore, a priori calculation of this critical force and consequently the critical particle concentration in colloidal systems was demonstrated by referring to the pressure at the liquid-to-solid transition in a hard sphere system (Alder transition).
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http://dx.doi.org/10.1016/j.jcis.2024.04.181 | DOI Listing |
Adv Mater
December 2024
Wuzhen Laboratory, Jiaxing, 314500, P. R. China.
Phase boundary is highly recognized for its capability in engineering various physical properties of ferroelectrics. Here, field-induced polarization rotation is reported in a high-performance (K, Na)NbO-based ferroelectric system at the rhombohedral-tetragonal phase boundary. First, the lattice structure is examined from both macroscopic and local scales, implementing Rietveld refinement and pair distribution function analysis, respectively.
View Article and Find Full Text PDFJ Phys Chem Lett
October 2024
Geochemical Research Center, Graduate School of Science, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-0033, Japan.
It is generally believed that ice crystal-to-crystal transitions do not occur below the glass-transition temperature. For instance, under compression, ice I becomes a metastable state but does not transform into other high-pressure ice crystals, and applying excessive pressure ends up causing its collapse into high-density amorphous ice (HDA). Here, we perform molecular dynamics (MD) simulations to demonstrate that a hydrogen-ordered form of cubic ice (ice Ic) transforms to a hydrogen-ordered form of ice IV without yielding HDA.
View Article and Find Full Text PDFPhys Rev E
July 2024
Departamento de Física, ICEx, Universidade Federal de Minas Gerais, C.P. 702, 30123-970 Belo Horizonte, Minas Gerais, Brazil.
We study a discrete-space model of active matter with excluded volume. Particles are restricted to the sites of a triangular lattice and can assume one of three orientations. Varying the density and noise intensity, Monte Carlo simulations reveal a variety of spatial patterns.
View Article and Find Full Text PDFPhys Rev E
July 2024
Department of Physics, Emory University, Atlanta, Georgia 30322, USA.
Flocking behavior is observed in biological systems from the cellular to superorganismal length scales, and the mechanisms and purposes of this behavior are objects of intense interest. In this paper, we study the collective dynamics of bovine sperm cells in a viscoelastic fluid. These cells appear not to spontaneously flock, but transition into a long-lived flocking phase after being exposed to a transient ordering pulse of fluid flow.
View Article and Find Full Text PDFNat Commun
August 2024
Laboratory of Nanomaterials & Nanomechanics, Department of Mechanical Engineering, City University of Hong Kong, Hong Kong, China.
Nanocrystalline metallic materials have the merit of high strength but usually suffer from poor ductility and rapid grain coarsening, limiting their practical application. Here, we introduce a core-shell nanostructure in a multicomponent alloy to address these challenges simultaneously, achieving a high tensile strength of 2.65 GPa, a large uniform elongation of 17%, and a high thermal stability of 1173 K.
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