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Hybrid Moiré Excitons and Trions in Twisted MoTe-MoSe Heterobilayers. | LitMetric

Hybrid Moiré Excitons and Trions in Twisted MoTe-MoSe Heterobilayers.

Nano Lett

Fakultät für Physik, Munich Quantum Center, and Center for NanoScience (CeNS), Ludwig-Maximilians-Universität München, Geschwister-Scholl-Platz 1, 80539 München, Germany.

Published: April 2024

We report experimental and theoretical studies of MoTe-MoSe heterobilayers with rigid moiré superlattices controlled by the twist angle. Using an effective continuum model that combines resonant interlayer electron tunneling with stacking-dependent moiré potentials, we identify the nature of moiré excitons and the dependence of their energies, oscillator strengths, and Landé -factors on the twist angle. Within the same framework, we interpret distinct signatures of bound complexes among electrons and moiré excitons in nearly collinear heterostacks. Our work provides a fundamental understanding of hybrid moiré excitons and trions in MoTe-MoSe heterobilayers and establishes the material system as a prime candidate for optical studies of correlated phenomena in moiré lattices.

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Source
http://dx.doi.org/10.1021/acs.nanolett.4c00541DOI Listing

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