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Hierarchical and reconfigurable interfibrous interface of bioinspired Bouligand structure enabled by moderate orderliness. | LitMetric

Hierarchical and reconfigurable interfibrous interface of bioinspired Bouligand structure enabled by moderate orderliness.

Sci Adv

Department of Chemistry, New Cornerstone Science Laboratory, Institute of Biomimetic Materials & Chemistry, Anhui Engineering Laboratory of Biomimetic Materials, Division of Nanomaterials & Chemistry, Hefei National Research Center for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei 230026, China.

Published: April 2024

AI Article Synopsis

  • Introducing a natural Bouligand structure into synthetic materials aims to create high-performance structural materials by enhancing load transfer through the interfibrous interface.
  • * A new hierarchical and reconfigurable interfibrous interface is designed using adaptable networked nanofibers, which enhances mechanical reinforcement and stability through dynamic adjustments.
  • * The system, demonstrated with bacterial cellulose nanofibers, shows improved strength and toughness due to the multiscale coupling of the interface and microstructure.

Article Abstract

Introducing natural Bouligand structure into synthetics is expected to develop high-performance structural materials. Interfibrous interface is critical to load transfer, and mechanical functionality of bioinspired Bouligand structure yet receives little attention. Here, we propose one kind of hierarchical and reconfigurable interfibrous interface based on moderate orderliness to mechanically reinforce bioinspired Bouligand structure. The interface imparted by moderate alignment of adaptable networked nanofibers hierarchically includes nanofiber interlocking and hydrogen-bonding (HB) network bridging, being expected to facilitate load transfer and structural stability through dynamic adjustment in terms of nanofiber sliding and HB breaking-reforming. As one demonstration, the hierarchical and reconfigurable interfibrous interface is constructed based on moderate alignment of networked bacterial cellulose nanofibers. We show that the resultant bioinspired Bouligand structural material exhibits unusual strengthening and toughening mechanisms dominated by interface-microstructure multiscale coupling. The proposed interfibrous interface enabled by moderate orderliness would provide mechanical insight into the assembly of widely existing networked nanofiber building blocks toward high-performance macroscopic bioinspired structural assemblies.

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Source
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC10997196PMC
http://dx.doi.org/10.1126/sciadv.adl1884DOI Listing

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