Because of the high efficiency of frequency conversion and beam-target coupling, a fourth harmonic (4) laser has a splendid application prospect in a high-power laser facility. The polarization smoothing (PS) crystal is preferably after the frequency conversion crystal to flexibly obtain the best uniformity illumination of the target. However, as a high irradiance 4 laser beam propagates through the PS crystal, the transverse stimulated Raman scattering (TSRS) effect of the PS crystal will be stronger, resulting in significant energy dissipation and crystal damage. This paper proposes a novel, to the best of our knowledge, fourth harmonic generation (FHG) scheme based on an orthogonal cascade of the DKDP crystals. This orthogonal cascaded FHG (OC-FHG) scheme employs two cascaded FHG crystals with orthogonal optical axes, and the PS crystal is in the middle. The PS crystal can rotate the polarization direction of the 2 laser by 90°, while the polarization direction of the 4 laser is maintained to a great extent. This OC-FHG scheme realizes the FHG by two steps, and the laser intensity at the PS crystal cuts down nearly 50%. The output intensity of the 4 laser can be increased from 1.8 / to about 3.6 / under the condition of effectively inhibiting the TSRS effect. Meanwhile, the output 4 laser contains two orthogonal polarized beams realizing in-beam polarization smoothing instantaneously. In addition, the novel FHG scheme can also have a high conversion efficiency and bandwidth tolerance.
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http://dx.doi.org/10.1364/AO.512229 | DOI Listing |
ACS Appl Mater Interfaces
January 2025
College of Optical, Mechanical and Electrical Engineering, Zhejiang A&F University, Lin'an 311300, China.
As a member of the chalcogenide family, NiSe exhibits a direct bandgap of 1.74 eV, making it a promising candidate for nonlinear optical devices. However, its potential in the near-infrared region of the telecommunication band has not been fully explored.
View Article and Find Full Text PDFSci Rep
December 2024
School of Earth Sciences, Northeast Petroleum University, Daqing, 163318, China.
Numerous gas-rich, low resistivity shale wells have been discovered in the Luzhou deep shale gas of Sichuan Basin, providing strong evidence that low-resistivity shale also holds significant potential for shale gas exploration. However, existing research has limited understanding of the mechanisms of low resistivity in shale, and the mechanisms by which low-resistivity influences gas content remain unclear. Here, we conducted X-ray diffraction analysis (XRD), total organic carbon (TOC) content, vitrinite reflectance (Ro), low-temperature N and CO adsorption experiments, methane isothermal adsorption experiments, nano-CT, laser Raman experiment, and well-logging curve to quantality evaluate the low resistivity shale formation mechanisms and explore the factors influencing gas content in low resistivity shale.
View Article and Find Full Text PDFAngew Chem Int Ed Engl
December 2024
Sichuan University, Department of Chemistry, wangjiang road NO.64, 610065, Chengdu, CHINA.
Enhancing the conversion efficiency of all-solid-state lasers through the rational design of crystal materials with superior linear and nonlinear optical (NLO) properties remains a formidable challenge. Herein, we present a novel approach to optimizing these properties in KBe2BO3F2 (KBBF)-analog crystals via functional group self-polymerization. This strategy led to the synthesis of two new optical crystals: noncentrosymmetric CsAs2O3Br and centrosymmetric CsAs4O6Br.
View Article and Find Full Text PDFPhys Rev E
November 2024
Institut für Theoretische Physik, Technikerstraße 21-A, Universität Innsbruck, A-6020 Innsbruck, Austria.
We analyze gravitaxis of a Brownian circle swimmer by deriving and analytically characterizing the experimentally measurable intermediate scattering function (ISF). To solve the associated Fokker-Planck equation, we use a spectral-theory approach, finding formal expressions in terms of eigenfunctions and eigenvalues of the overdamped-noisy-driven pendulum problem. We further perform a Taylor series of the ISF in the wavevector to extract the cumulants up to the fourth order.
View Article and Find Full Text PDFReducing the repetition rate is one of the effective ways to increase the peak-power of the mode-locked pulses. However, for a vertical-external-cavity surface-emitting laser (VECSEL), the carrier lifetime in the nanosecond regime limits the further reduction of the pulse repetition rate, or in other words, limits the average output power of the mode-locked laser at low repetition rates, and ultimately restricts the peak-power of the pulses. This work uses a specially designed saturable Bragg reflector to start the mode-locking, and both low repetition rate and high average power are achieved simultaneously in a passively mode-locked VECSEL.
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