The occurrence and ecological risks of 16 polycyclic aromatic hydrocarbons (PAHs) in different types of urban road runoff in Beijing during two typical rainfall events were studied. The average concentration of PAHs in road runoff particulate was in the order of Guanyuanqiao Road (ring road, 15,175 ng/L) > Huayuanqiao Road (primary road, 4,792 ng/L) > Dongcheng Alley (alley, 4,774 ng/L) > Nansihuan Viaduct (viaduct, 770 ng/L), much higher than dissolved PAHs. The total concentration of ∑16PAHs decreased with runoff scouring. Rainfall conditions and the accumulation of PAHs in the early rainfall period show a significant impact on PAHs pollution. The event mean concentration range of PAHs is 674-21,596 ng/L, following in the order of ring road > primary road > alley > viaduct. The proportion of four-ring PAHs was the highest. The first flush effect of PAHs is found in both rainfall events, and the effect of different ring PAHs is relatively similar. The content of PAHs is positively correlated with the amount of total organic carbon and suspended substance in runoff (r> 0.72). The ecological risk assessment indicated that PAHs in road runoff except viaduct road corresponded to high risk.
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http://dx.doi.org/10.2166/wst.2024.035 | DOI Listing |
J Environ Manage
December 2024
Earth System Science Interdisciplinary Center, University of Maryland, College Park, 5825 University Research Ct, College Park, MD, 20740, USA.
Urbanization increases the extent of impervious surfaces, runoff, sediment, and nutrient loadings downstream, leading to the deterioration of urban surface waters. During pollutant wash-off from urban surfaces, the peak concentration of pollutants typically occurs after the rainfall peak. However, current urban wash-off models do not consider this time delay, assuming that the effect of rainfall on the wash-off process is immediate.
View Article and Find Full Text PDFMar Pollut Bull
December 2024
BCSIR Laboratories Dhaka, Bangladesh Council of Scientific and Industrial Research (BCSIR), Dhaka 1205, Bangladesh; Cental Analytical Research Facilities (CARF), Bangladesh Council of Scientific and Industrial, Dr Qudrat-i-Khuda Road, Dhanmondi, Dhaka 1205, Bangladesh. Electronic address:
The Payra River, cicual for fish breeding, feeding and nursery in coastal Bangladesh, faces heavy contamination from industrial activities, agricultural runoff and poor waste management. This study used ICP-MS to assess metal contamination levels, risk status and potential sources in river sediment. The findings showed that the mean concentrations (mg/kg) of metals followed the decreasing order: Mn (434.
View Article and Find Full Text PDFJ Environ Manage
December 2024
Key Laboratory of Agro-ecological Processes in Subtropical Region, Institute of Subtropical Agriculture, Chinese Academy of Sciences, Changsha 410125, China; Guangxi Key Laboratory of Karst Ecological Processes and Services, Huanjiang Observation and Research Station of Karst Ecosystems, Chinese Academy of Sciences, Huanjiang 547100, Guangxi, China. Electronic address:
In karst landscapes, where sustainable water management is increasingly challenged by drought-induced water scarcity, the adoption of road-based rainwater harvesting (RBWH) systems has emerged as a promising solution for improving water accessibility. Despite the growing implementation of such systems, the effectiveness of many RBWH projects in karst terrains remains suboptimal due to an inadequate understanding of runoff generation mechanisms associated with hilly road networks. This study focuses on quantifying the contributions of intercepted surface runoff (SR) and soil-epikarst lateral flow (SEF) from a newly exposed road-cut slope in a dolomite hillslope, with data collected across 156 rainfall events from May 2019 to May 2022.
View Article and Find Full Text PDFEnviron Sci Technol
December 2024
School of Chemistry and Biological Engineering, University of Science and Technology Beijing, Beijing 100083, China.
Tire and road wear particles (TRWPs) are an appreciable source of microplastics (MPs); however, knowledge of their large-scale occurrence and mass flux based on robust sampling and quantification is limited. Herein, the first city-wide survey of TRWPs across environmental compartments (road dust, snowbank, water, and sediment from rivers and lakes) along four ring roads (beltways) in Beijing was performed. TRWP concentrations ( = 74) were quantified using bonded-sulfur as a marker to reveal the city-wide spatial distributions and adopted to establish a framework estimating TRWP emission factors (EFs) and mass flux from generation to remote atmospheric, terrestrial, and aquatic transport.
View Article and Find Full Text PDFWater Res
December 2024
School of Environment, Nanjing Normal University, Jiangsu Province Engineering Research Center of Environmental Risk Prevention and Emergency Response Technology, Jiangsu Engineering Lab of Water and Soil Eco-remediation, Wenyuan Road 1, Nanjing 210023, PR China. Electronic address:
Coupling of iron-carbon can form a mixotrophic denitrification and is regarded as a promising solution for purifying nitrate-rich agricultural runoff. However, its prevalence and efficacy of the synergistic augmentation of nitrogen elimination and net NO sinks remain crucial knowledge gaps in ecological ditches (eco-ditches). Here, we investigated the underlying variability mechanisms by implementing sponge iron (sFe)-coupled Iris hexagonus (IH)- or Myriophyllum aquaticum (MA)-derived biochar produced via microwave-assisted (MW) pyrolysis and conventional pyrolysis.
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