Measurement of tritium surface contamination is important for tritium related facilities, especially for fusion devices. A novel detector has been designed for tritium surface contamination measurements based on CaF(Eu) sheet and Microchannel plate photomultiplier tube (MCP-PMT). Self-coincidence technology has been introduced to obtain lower detection limit by diminishing the background noise caused by γ-rays and hot electrons. Performance of the detector was optimized by specifying the key parameters including the distance of the scintillator and sample, the thickness of light guide, the number of annular electrodes et al., using Monte Carlo method. Results indicate that detection efficiency of 49.4 % and the response deviations at different positions less than 0.5 % could be achieved. The detection limit of tritium under the simulation conditions is 0.09 Bq/cm and 0.03 Bq/cm when the counting time is 10 s and 60 s, respectively.
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http://dx.doi.org/10.1016/j.apradiso.2024.111200 | DOI Listing |
Anal Chem
January 2025
Department of Bioproducts and Biosystems, School of Chemical Engineering, Aalto University, 00076 Aalto, Finland.
Accurately quantifying specific proteins from complex mixtures like cell lysates, for example, during in vivo studies, is difficult, especially for aggregation-prone proteins. Herein, we describe the development of a specific protein quantification method that combines a solid-state dot blot approach with radiolabel detection via liquid scintillation counting. The specific detection with high sensitivity is achieved by using the Twin-Strep protein affinity tag and tritium-labeled Strep-TactinXT probe.
View Article and Find Full Text PDFJ Environ Radioact
December 2024
Graduate School of Human Environment, Osaka Sangyo University, Osaka, 5748530, Japan.
Tritium, a radioactive isotope produced naturally through cosmic radiation interactions and anthropogenically through nuclear weapons testing, poses potential environmental risks, particularly within the water cycle. This study measured tritium concentrations in surface water across Thailand to establish a baseline dataset for monitoring potential contamination from nuclear activities and accidents. Surface water samples were collected from 14 large reservoirs during the wet season in October 2023 and the dry season in February 2024, providing a total of 28 samples.
View Article and Find Full Text PDFPhys Chem Chem Phys
December 2024
National Energy Technology Laboratory, 626 Cochran Mill Road, Pittsburgh, PA 15236, USA.
The nickel-plated zircaloy-4 is used as a tritium (H) getter in the tritium-producing burnable absorber rods (TPBARs) to capture H produced in the Li-riched annular γ-LiAlO pellet under neutron irradiation. The experimental data and our previous theoretical results showed that the H species produced from the γ-LiAlO pellet were mainly H and HO. These H species diffuse from the surface of the LiAlO pellet across vacuum to the nickel-plated zircaloy-4 getter and then further diffuse into the getter to chemically form metal hydrides.
View Article and Find Full Text PDFSci Total Environ
December 2024
College of Life Science, Northeast Forestry University, No. 26, Hexing Road, Harbin 150040, China. Electronic address:
Appl Radiat Isot
November 2024
Research Institute of Electronics, Shizuoka University, 3-5-1 Johoku, Chuo-ku, Hamamatsu City, Shizuoka, 432-8011, Japan.
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