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Theory for magnetic impurity modes in two-dimensional van der Waals ferromagnetic films. | LitMetric

Theory for magnetic impurity modes in two-dimensional van der Waals ferromagnetic films.

J Phys Condens Matter

Department of Physics and Astronomy, University of Western Ontario, London, Ontario N6A 3K7, Canada.

Published: February 2024

AI Article Synopsis

Article Abstract

A spin-wave analysis is developed to calculate the energies of the localized excitations occurring in two-dimensional ferromagnetic van der Waals monolayers when a substitutional magnetic impurity is introduced. The magnetic ions lie on a bipartite honeycomb lattice (similar to that for graphene) and the theory includes the effects of both Ising anisotropy and single-ion anisotropy to stabilize the magnetic ordering perpendicular to the atomic plane at low temperatures. A Dyson-equation formalism, together with the spin-dependent Green's functions derived for van der Waals monolayers, is employed to evaluate the existence conditions and energies for the impurity modes, which lie above the band of spin-wave states of the pure host material. For realistic parameter values it is found that typically two impurity modes may exist, depending on the spin quantum number for the magnetic impurity atom. Numerical applications are made to CrIand CrGeTeas the host materials.

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http://dx.doi.org/10.1088/1361-648X/ad2671DOI Listing

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