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Catalytic conversion of biomass-derived 5-hydroxymethylfurfural to 5-hydroxymethyl-2-furancarboxylic acid using novel cobalt-based MOF in the presence of deep eutectic solvents.
Sci Rep
December 2024
Department of Organic Chemistry, Faculty of Chemistry, University of Mazandaran, Babolsar, 47416-95447, Iran.
The oxidation of 5-HMF to HMFCA is an important yet complex process, as it generates high-value chemical intermediates. Achieving this transformation efficiently requires the development of non-precious, highly active catalysts derived from renewable biomass sources. In this work, we introduce UoM-1 (UoM, University of Mazandaran), a novel cobalt-based metal-organic framework (Co-MOF) synthesized using a simple one-step ultrasonic irradiation method.
View Article and Find Full Text PDFResearch on the evolutionary characteristics and mechanism of production-living-ecological space in Shanxi Province, China.
Sci Rep
December 2024
School of Economics and Management, Taiyuan Normal University, Taiyuan, 030619, China.
An investigation of the evolutionary characteristics and internal driving mechanisms of territorial space since the reform and opening up is essential. The study will guide the orderly development and rational layout of territorial space, as well as achievement transformation and high-quality development in Shanxi Province. We used land use data from 1980 to 2020, which was divided into four periods, to examine the changes in production-living-ecological spatial pattern in Shanxi Province.
View Article and Find Full Text PDFOn machine learnability of local contributions to interatomic potentials from density functional theory calculations.
Sci Rep
December 2024
Department of Physics, Shahid Beheshti University, Tehran, 1983969411, Iran.
Machine learning interatomic potentials, as a modern generation of classical force fields, take atomic environments as input and predict the corresponding atomic energies and forces. We challenge the commonly accepted assumption that the contribution of an atom can be learned from the short-range local environment of that atom. We employ density functional theory calculations to quantify the decay of the induced electron density and electrostatic potential in response to local perturbations throughout insulating, semiconducting and metallic samples of different dimensionalities.
View Article and Find Full Text PDFEffects of water-fertiliser coupling on the photosynthesis and quality of Lycium barbarum based on predicted crop evapotranspiration (ET).
Sci Rep
December 2024
School of Civil and Hydraulic Engineering, Ningxia University, Yinchuan, Ningxia, 750021, China.
Lycium barbarum is an important economic crop in the arid region of Northwest China, and the regulation of irrigation and fertilisation is an important way to improve the quality and yield of Lycium barbarum. To explore the effects of water-fertiliser coupling on photosynthesis, quality and yield of Lycium barbarum under irrigation methods based on predicted crop evapotranspiration (ET), ET was calculated via reference evapotranspiration (ET) predicted on the basis of public weather forecasts, and the irrigation water volume was determined as a proportion of this ET. A field experiment was conducted via a completely randomised experimental design with five irrigation water volumes (W0 (100% ET), W1 (90% ET), W2 (80% ET), W3 (70% ET) and W4 (65% ET)) and three fertiliser application rates (high fertiliser (FH), medium fertiliser (FM) and low fertiliser (FL)).
View Article and Find Full Text PDFUnderstanding the association between urban noise and nighttime light in China.
Sci Rep
December 2024
School of Architecture and Urban-Rural Planning, Fuzhou University, Fuzhou, 350108, China.
Nighttime light data partially reflects the process of urban modernization and its reaction to urban scale, but its correlation with noise remains unclear, especially over a long-term time series, remains unclear. To address this gap, we examine 31 provincial capital cities and municipalities in China as the study area, utilizing noise monitoring data and nighttime light data to explore their relationship in urban areas from 2012 to 2021. The results show that: (1) During the study period, the regional environmental noise and night light index of 31 major cities exhibited a consistent upward trend, with the average equivalent sound level of environmental noise in most urban areas fluctuating between 50.
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