Nematic Spin Correlations Pervading the Phase Diagram of FeSe_{1-x}S_{x}.

Phys Rev Lett

Center for Advanced Quantum Studies and Department of Physics, Beijing Normal University, Beijing 100875, People's Republic of China.

Published: January 2024

AI Article Synopsis

  • The study uses resonant inelastic x-ray scattering (RIXS) to analyze spin excitations in uniaxially-strained and unstrained FeSe_{1-x}S_{x} samples, finding that spin excitations show minimal variation with sulfur doping.
  • RIXS results indicate that a high-energy spin-excitation anisotropy persists across a range of doping levels (0≤x≤0.21) and remains significant at temperatures above 200 K, peaking near the nematic quantum critical doping point (x_{c}≈0.17).
  • The findings suggest that spin fluctuations are crucial for electronic nematicity and illustrate how uniaxial strain can modulate spin excitations in materials with strong magnet

Article Abstract

We use resonant inelastic x-ray scattering (RIXS) at the Fe-L_{3} edge to study the spin excitations of uniaxial-strained and unstrained FeSe_{1-x}S_{x} (0≤x≤0.21) samples. The measurements on unstrained samples reveal dispersive spin excitations in all doping levels, which show only minor doping dependence in energy dispersion, lifetime, and intensity, indicating that high-energy spin excitations are only marginally affected by sulfur doping. RIXS measurements on uniaxial-strained samples reveal that the high-energy spin-excitation anisotropy observed previously in FeSe is also present in the doping range 0200  K in x=0.18 and reaches a maximum around the nematic quantum critical doping (x_{c}≈0.17). Since the spin-excitation anisotropy directly reflects the existence of nematic spin correlations, our results indicate that high-energy nematic spin correlations pervade the regime of nematicity in the phase diagram and are enhanced by the nematic quantum criticality. These results emphasize the essential role of spin fluctuations in driving electronic nematicity and highlight the capability of uniaxial strain in tuning spin excitations in quantum materials hosting strong magnetoelastic coupling and electronic nematicity.

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http://dx.doi.org/10.1103/PhysRevLett.132.016501DOI Listing

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