This article covers selected properties of organic-inorganic thin films of hybrid perovskites with the summary formulas CHNHI, where = Pb, Cd, Ge, Sn, Zn. The paper discusses not only the history, general structure, applications of perovskites and the basics of the theory of nonlinear optics, but also the results of experimental research on their structural, spectroscopic, and nonlinear optical properties. The samples used in all presented studies were prepared in the physical vapor deposition process by using co-deposition from two independent thermal sources containing the organic and inorganic parts of individual perovskites. Ultimately, thin layers with a thickness of the order of nanometers were obtained on glass and crystalline substrates. Their structural properties were characterized by atomic force microscopy imaging. Spectroscopic tests were used to confirm the tested films' transmission quality and determine previously unknown physical parameters, such as the absorption coefficient and refractive index. Experimental results of the nonlinear optical properties were obtained by studying the second and third harmonic generation processes and using initial sample polarization in the so-called Corona poling process. The obtained experimental results allowed us to determine the second- and third-order nonlinear optical susceptibility of the tested materials.
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http://dx.doi.org/10.3390/nano14010050 | DOI Listing |
Nano Lett
January 2025
Department of Electrical and Computer Engineering, Northwestern University, Evanston, Illinois 60208, United States.
Metasurfaces supporting narrowband resonances are of significant interest in photonics for molecular sensing, quantum light source engineering, and nonlinear photonics. However, many device architectures rely on large refractive index dielectric materials and lengthy fabrication processes. In this work, we demonstrate quasi-bound states in the continuum (quasi-BICs) using a polymer metasurface exhibiting experimental quality factors of 305 at visible wavelengths.
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January 2025
Research Laboratory of Electronics, MIT, Cambridge, MA, USA.
Three-dimensional subcellular imaging is essential for biomedical research, but the diffraction limit of optical microscopy compromises axial resolution, hindering accurate three-dimensional structural analysis. This challenge is particularly pronounced in label-free imaging of thick, heterogeneous tissues, where assumptions about data distribution (e.g.
View Article and Find Full Text PDFLight Sci Appl
January 2025
Laboratoire Matériaux et Phénomènes Quantiques, Université Paris Cité and CNRS, Paris, 75013, France.
Vortex beams are currently drawing a great deal of interest, from fundamental research to several promising applications. While their generation in bulky optical devices limits their use in integrated complex systems, metasurfaces have recently proven successful in creating optical vortices, especially in the linear regime. In the nonlinear domain, of strategic importance for the future of classical and quantum information, to date orbital angular momentum has only been created in qualitative ways, without discussing discrepancies between design and experimental results.
View Article and Find Full Text PDFLight Sci Appl
January 2025
Spin-Optics laboratory, St. Petersburg State University, St. Petersburg, 198504, Russia.
We introduce a novel neuromorphic network architecture based on a lattice of exciton-polariton condensates, intricately interconnected and energized through nonresonant optical pumping. The network employs a binary framework, where each neuron, facilitated by the spatial coherence of pairwise coupled condensates, performs binary operations. This coherence, emerging from the ballistic propagation of polaritons, ensures efficient, network-wide communication.
View Article and Find Full Text PDFScience
January 2025
Department of Electrical, Computer and Energy Engineering, University of Colorado Boulder, Boulder, CO, USA.
Optical frequency combs have enabled unique advantages in broadband, high-resolution spectroscopy and precision interferometry. However, quantum mechanics ultimately limits the metrological precision achievable with laser frequency combs. Quantum squeezing has led to significant measurement improvements with continuous wave lasers, but experiments demonstrating metrological advantage with squeezed combs are less developed.
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