The anomalous Hall effect (AHE) is an important transport signature revealing topological properties of magnetic materials and their spin textures. Recently, MnBiTe has been demonstrated to be an intrinsic magnetic topological insulator. However, the origin of its intriguing AHE behaviors remains elusive. Here, we demonstrate the Berry curvature-dominated intrinsic AHE in wafer-scale MnBiTe films. By applying back-gate voltages, we observe an ambipolar conduction and transition in ∼7-layer MnBiTe, where a quadratic relation between the AHE resistance and longitudinal resistance suggests its intrinsic AHE nature. In particular, for ∼3-layer MnBiTe, the AHE sign can be tuned from pristine negative to positive. First-principles calculations unveil that such an AHE reversal originated from the competing Berry curvature between oppositely polarized spin-minority-dominated surface states and spin-majority-dominated inner bands. Our results shed light on the underlying physical mechanism of the intrinsic AHE and provide new perspectives for the unconventional sign-tunable AHE.
Download full-text PDF |
Source |
---|---|
http://dx.doi.org/10.1021/acs.nanolett.3c02926 | DOI Listing |
J Phys Condens Matter
January 2025
Department of Physics, Indian Institute of Technology Delhi, Hauz Khas, New Delhi 110016, India.
Time-reversal symmetry breaking of a topological insulator phase generates zero-field edge modes which are the hallmark of the quantum anomalous Hall effect (QAHE) and of possible value for dissipation-free switching or non-reciprocal microwave devices. But present material systems exhibiting the QAHE, such as magnetically doped bismuth telluride and twisted bilayer graphene, are intrinsically unstable, limiting their scalability. A pristine magnetic oxide at the surface of a TI would leave the TI structure intact and stabilize the TI surface, but epitaxy of an oxide on the lower-melting-point chalcogenide presents a particular challenge.
View Article and Find Full Text PDFPhys Rev Lett
November 2024
School of Physical Science and Technology, ShanghaiTech University, Shanghai 201210, China.
Generally, the dissipationless Hall effect in solids requires time-reversal symmetry breaking (TRSB), where TRSB induced by external magnetic field results in the ordinary Hall effect, while TRSB caused by spontaneous magnetization gives rise to the anomalous Hall effect (AHE) which scales with the net magnetization. The AHE is therefore not expected in antiferromagnets with vanishing small magnetization. However, large AHE was recently observed in certain antiferromagnets with noncollinear spin structure and nonvanishing Berry curvature.
View Article and Find Full Text PDFACS Nano
December 2024
Department of Physics and Astronomy, Birck Nanotechnology Center, and Purdue Quantum Science and Engineering Institute, Purdue University, West Lafayette, Indiana 47907, United States.
Two-dimensional (2D) magnets, as an important member of the 2D material family, have emerged as a promising platform for spintronic devices. Herein, we report the chemical vapor deposition (CVD) growth of highly crystalline submillimeter-scale self-intercalated metallic 2D ferromagnetic (FM) trigonal chromium telluride (CrTe) flakes on inert mica substrates. Through magneto-optical and magnetotransport measurements, we unveil the exceptional magnetic properties of these 2D flakes.
View Article and Find Full Text PDFAdv Sci (Weinh)
January 2025
Department of Physics, University at Buffalo, The State University of New York, Buffalo, NY, 14226, USA.
Covalent 2D magnets such as CrTe, which feature self-intercalated magnetic cations located between monolayers of transition-metal dichalcogenide material, offer a unique platform for controlling magnetic order and spin texture, enabling new potential applications for spintronic devices. Here, it is demonstrated that the unconventional anomalous Hall effect (AHE) in CrTe, characterized by additional humps and dips near the coercive field in AHE hysteresis, originates from an intrinsic mechanism dictated by the self-intercalation. This mechanism is distinctly different from previously proposed mechanisms such as topological Hall effect, or two-channel AHE arising from spatial inhomogeneities.
View Article and Find Full Text PDFSmall
January 2025
Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing, 100190, China.
Creating a heterostructure by combining two magnetically and structurally distinct ruthenium oxides is a crucial approach for investigating their emergent magnetic states and interactions. Previously, research has predominantly concentrated on the intrinsic properties of the ferromagnet SrRuO and recently discovered altermagnet RuO solely. Here, the study engineers an ultrasharp sublattice-matched heterointerface using pseudo-cubic SrRuO and rutile RuO, conducting an in-depth analysis of their spin interactions.
View Article and Find Full Text PDFEnter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!