Correlated Electronic Structure of La_{3}Ni_{2}O_{7} under Pressure.

Phys Rev Lett

Department of Physics, University of Fribourg, 1700 Fribourg, Switzerland.

Published: November 2023

Recently, superconductivity with a T_{c} up to 78 K has been reported in bulk samples of the bilayer nickelate La_{3}Ni_{2}O_{7} at pressures above 14 GPa. Important theoretical tasks are the formulation of relevant low-energy models and the clarification of the normal state properties. Here, we study the correlated electronic structure of the high-pressure phase in a four-orbital low-energy subspace using different many-body approaches: GW, dynamical mean field theory (DMFT), extended DMFT (EDMFT) and GW+EDMFT, with realistic frequency-dependent interaction parameters. The nonlocal correlation and screening effects captured by GW+EDMFT result in an instability toward the formation of charge stripes, with the 3d_{z^{2}} as the main active orbital. We also comment on the potential relevance of the rare-earth self-doping pocket, since hole doping suppresses the ordering tendency.

Download full-text PDF

Source
http://dx.doi.org/10.1103/PhysRevLett.131.206501DOI Listing

Publication Analysis

Top Keywords

correlated electronic
8
electronic structure
8
structure la_{3}ni_{2}o_{7}
4
la_{3}ni_{2}o_{7} pressure
4
pressure superconductivity
4
superconductivity t_{c}
4
t_{c} 78 k
4
78 k reported
4
reported bulk
4
bulk samples
4

Similar Publications

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!