Dependence of the Glass Transition and Jamming Densities on Spatial Dimension.

Phys Rev Lett

Theoretical Sciences Unit and School of Advanced Materials, Jawaharlal Nehru Centre for Advanced Scientific Research, Jakkur Campus, 560064 Bengaluru, India.

Published: October 2023

We investigate the dynamics of soft sphere liquids through computer simulations for spatial dimensions from d=3 to 8, over a wide range of temperatures and densities. Employing a scaling of density-temperature-dependent relaxation times, we precisely identify the density ϕ_{0}, which marks the ideal glass transition in the hard sphere limit, and a crossover from sub- to super-Arrhenius temperature dependence. The difference between ϕ_{0} and the athermal jamming density ϕ_{J}, small in 3 and 4 dimensions, increases with dimension, with ϕ_{0}>ϕ_{J} for d>4. We compare our results with recent theoretical calculations.

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http://dx.doi.org/10.1103/PhysRevLett.131.168202DOI Listing

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