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We report on the experimental development of short-tapered chalcogenide-glass rods for mid-infrared supercontinuum generation. Multi-octave spectral broadening of femtosecond laser pulses is demonstrated from 1.6 to 15.6 µm in a 5-cm-long tapered GeSeTe rod with a waist diameter of 25 µm. Despite the multimode nature of the optical waveguide used, this work clearly shows the potential of such simple post-processed rods for advancing fiber SC sources with infrared glasses, thereby unlocking new possibilities in terms of coupling efficiency, spectral coverage, and output power.
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http://dx.doi.org/10.1364/OL.501036 | DOI Listing |
Appl Spectrosc
December 2024
Department of Electrical and Photonics Engineering, Technical University of Denmark, Kongens Lyngby, Denmark.
Combining near-infrared (NIR) and mid-infrared (MIR) spectroscopy to cover both the fundamental and overtone combination molecular vibrational resonances allows more robust analytical methods to be used, such as two-dimensional correlation spectroscopy. However, due to the strong differences in molar absorption coefficients and transparency of the optical material, it is inherently difficult to perform NIR and MIR spectroscopy on aqueous samples using a single instrument. Combining spectra from different instruments and sample presentations can result in unwanted spectral variations, which can influence the prediction models and mitigate the advantages of the combination approaches.
View Article and Find Full Text PDFThis study demonstrates the potential to generate a soft x-ray single-cycle attosecond pulse using a single-cycle mid-infrared pulse from advanced dual-chirped optical parametric amplification (DC-OPA). A super continuum high harmonic (HH) spectrum was generated in argon (80-160 eV) and neon (150-270 eV). The experimental spectra reasonably agree with those calculated by the strong-field approximation model and Maxwell's equations.
View Article and Find Full Text PDFA silica volume Bragg grating (VBG) is used to filter the light of a mid-infrared (mid-IR) supercontinuum laser. The VBG with a 7 µm period was inscribed with 800 nm pulses with a 100 fs duration and the phase-mask technique over a glass thickness of 3 mm. Despite silica's absorption, the VBG allows obtaining a narrowband light source tunable from 2.
View Article and Find Full Text PDFSupercontinuum sources based on intrapulse difference frequency generation (IDFG) from mode-locked lasers open new opportunities in mid-infrared gas spectroscopy. These sources provide high power and ultra-broadband spectral coverage in the molecular fingerprint region with very low relative intensity noise. Here, we demonstrate the performance of such a light source in combination with a multipass cell and a custom-built Fourier transform spectrometer (FTS) for multispecies trace gas detection.
View Article and Find Full Text PDFHere, we demonstrate a compact and efficient high-power mid-infrared supercontinuum (MIR-SC) laser source based on a tunable noise-like pulse (NLP) fiber laser system and a short section of single-mode germania-core fiber (GCF). The NLP all-polarization-maintaining fiber laser system can deliver the maximum output power of ∼30.6 W and a broadband spectrum (∼1.
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