Soil contamination is an environmental issue due to increasing anthropogenic activities. Existing processes for soil remediation suffer from long treatment time and lack generality because of different sources, occurrences, and properties of pollutants. Here, we report a high-temperature electrothermal process for rapid, water-free remediation of multiple pollutants in soil. The temperature of contaminated soil with carbon additives ramps up to 1000 to 3000 °C as needed within seconds via pulsed direct current input, enabling the vaporization of heavy metals like Cd, Hg, Pb, Co, Ni, and Cu, and graphitization of persistent organic pollutants like polycyclic aromatic hydrocarbons. The rapid treatment retains soil mineral constituents while increases infiltration rate and exchangeable nutrient supply, leading to soil fertilization and improved germination rates. We propose strategies for upscaling and field applications. Techno-economic analysis indicates the process holds the potential for being more energy-efficient and cost-effective compared to soil washing or thermal desorption.
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http://dx.doi.org/10.1038/s41467-023-41898-z | DOI Listing |
ACS Appl Mater Interfaces
December 2024
Institute of Chemical Engineering Sciences, Foundation of Research and Technology- Hellas (FORTH/ICE-HT), Stadiou Street, Platani, Patras 26504, Greece.
Due to their outstanding electrical and thermal properties, graphene and related materials have been proposed as ideal candidates for the development of lightweight systems for thermoelectric applications. Recently, the nanolaminate architecture that entails alternation of continuous graphene monolayers and ultrathin polymer films has been proposed as an efficient route for the development of composites with impressive physicochemical properties. In this work, we present a novel layer-by-layer approach for the fabrication of highly ordered, flexible, heat-resistant, and electrically conductive freestanding graphene/polymer nanolaminates through alternating Marangoni-driven self-assembly of reduced graphene oxide (rGO) and poly(ether imide) (PEI) films.
View Article and Find Full Text PDFInt J Biol Macromol
December 2024
State Key Laboratory for New Textile Materials and Advanced Processing Technology, School of Materials Science and Engineering, Wuhan Textile University, Wuhan 430200, PR China. Electronic address:
The design of multifunctional, high-performance wearable heaters utilizing textile substrates has garnered increasing attention, particularly in the development of body temperature and health monitoring devices. However, fabricating these multifunctional wearable heaters while simultaneously ensuring flexibility, air permeability, Joule heating performance, electromagnetic interference (EMI) shielding and antibacterial properties remains a significant challenge. This study utilizes phase transition lysozyme (PTL) film-mediated electroless deposition (ELD) technology to deposit silver nanoparticles (Ag NPs) on the cotton fabrics surface in a mild aqueous solution at room temperature, thereby constructing a wearable heater with long-term stability, high conductivity, and exceptional photothermal properties.
View Article and Find Full Text PDFAdv Mater
December 2024
State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering, Donghua University, Shanghai, 201620, China.
Stretchable fibers with high conductivity are vital components for smart textiles and wearable electronics. However, embedding solid conductive materials in polymers significantly reduces conductive pathways when stretched, causing a sharp drop in conductivity. Here, a stretchable metastructured fiber with dynamic liquid metal-microfiber interlocking interface is reported to realize highly conductive yet ultrastable conductance.
View Article and Find Full Text PDFPolymers (Basel)
November 2024
Shaanxi Collaborative Innovation Center of Green Intelligent Printing and Packaging, Xi'an University of Technology, Xi'an 710054, China.
Micromachines (Basel)
October 2024
Department of Electrical Engineering, École de Technologie Supérieure, Université du Québec, Montréal, QC H3C 1K3, Canada.
Electrothermal actuators are highly advantageous for microelectromechanical systems (MEMS) due to their capability to generate significant force and large displacements. Despite these benefits, their application in reconfigurable conduction line switches is limited, particularly when employing commercial processes. In DC MEMS switches, electrothermal actuators require electrical insulation between the biasing voltage and the transmission line to prevent interference and maintain the integrity of the switch.
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