Helical dichroism (HD) utilizing unbounded orbital angular momentum degree of freedom, has provided an important means of exploring chiral effects in diverse wave systems, surpassing the two-state constraint in circular dichroism that relies on intrinsic spin. However, the naturally feeble chiral signals that arise during wave-matter interactions pose significant challenges to the effective enlargement of HD. Here, we introduce a new paradigm for realizing maximum HD through non-Hermitian gradient metasurfaces by engineering a chiral exceptional point (EP) in intrinsic topological charge. The non-Hermitian gradient metasurfaces are empowered by the asymmetric coupling feature at the EP, enabling flexible construction to realize versatile chirality control in extreme circumstances where one chiral vortex is totally reflected and the opposite counterpart is completely absorbed or transmitted into the customized vortex modes. As the manifestation of the maximum HD, we present the first experimental demonstration of perfect chirality-selected vortex transmission in acoustics. Our findings open new venues to achieve maximum chirality and explore chiral physics of wave-matter interactions, which can boost many vortical applications in asymmetric chirality manipulation, one-way propagation, and information multiplexing.
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http://dx.doi.org/10.1016/j.scib.2023.09.028 | DOI Listing |
J Chem Phys
October 2024
Department of Chemistry and Engineering Research Center of Advanced Rare-Earth Materials of Ministry of Education, Tsinghua University, Beijing 100084, China.
The matrix product state (MPS) Ansatz offers a promising approach for finding the ground state of molecular Hamiltonians and solving quantum chemistry problems. Building on this concept, the proposed technique of quantum circuit MPS (QCMPS) enables the simulation of chemical systems using a relatively small number of qubits. In this study, we enhance the optimization performance of the QCMPS Ansatz by employing the variational quantum imaginary time evolution (VarQITE) approach.
View Article and Find Full Text PDFSci Bull (Beijing)
November 2023
College of Physics, Nanjing University of Aeronautics and Astronautics, Nanjing 211106, China; Key Laboratory of Aerospace Information Materials and Physics, Ministry of Industry and Information Technology, Nanjing 211106, China; State Key Laboratory of Mechanics and Control for Aerospace Structures, Nanjing University of Aeronautics and Astronautics, Nanjing 210016, China. Electronic address:
Helical dichroism (HD) utilizing unbounded orbital angular momentum degree of freedom, has provided an important means of exploring chiral effects in diverse wave systems, surpassing the two-state constraint in circular dichroism that relies on intrinsic spin. However, the naturally feeble chiral signals that arise during wave-matter interactions pose significant challenges to the effective enlargement of HD. Here, we introduce a new paradigm for realizing maximum HD through non-Hermitian gradient metasurfaces by engineering a chiral exceptional point (EP) in intrinsic topological charge.
View Article and Find Full Text PDFNat Commun
September 2023
The Czech Academy of Sciences, Institute of Scientific Instruments, Královopolská 147, 612 64, Brno, Czech Republic.
We explore, experimentally and theoretically, the emergence of coherent coupled oscillations and synchronization between a pair of non-Hermitian, stochastic, opto-mechanical oscillators, levitated in vacuum. Each oscillator consists of a polystyrene microsphere trapped in a circularly polarized, counter-propagating Gaussian laser beam. Non-conservative, azimuthal forces, deriving from inhomogeneous optical spin, push the micro-particles out of thermodynamic equilibrium.
View Article and Find Full Text PDFChem Commun (Camb)
April 2022
Department of Chemistry, KU Leuven, Celestijnenlaan 200F, B-3001 Leuven, Belgium.
Unlike the ideal circular whispering gallery cavities, those without mirror symmetry intrinsically support resonant modes exhibiting chirality which indicates an imbalance between clockwise and counterclockwise wave components. In extreme cases, nearly degenerate pairs of copropagating modes can be found around the chiral exceptional points (EPs) in parameter spaces. The chiral EPs have been studied in various schemes; however, most attention has been focused on the cases with piecewise constant or periodic refractive index profiles.
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