Spatiotemporal distribution of air pollutants during a heat wave-induced forest fire event in Uttarakhand.

Prevailing dry conditions and rainfall deficit during the spring season in North India led to heat wave conditions which resulted in widespread and intense forest fire events in the Himalayan state of Uttarakhand during April 16-30, 2022. A total of 7589 active fires were detected by VIIRS during the second half of April 2022 compared to 1558 during the first half. The TROPOMI observed total column values of CO and NO increased by 4.4% and 11.7%, respectively during April 16-30, 2022 with respect to April 1-15, 2022. A noticeable increase in surface level concentration of trace gases was also observed at Dehradun. In situ measurements of CO, NO, and O during April 16-30, 2022 show an increase of 133, 35, and 6% compared to previous year observations during the same period. Weather Research and Forecasting model with chemistry (WRF-Chem) is utilized to quantitatively estimate the contribution of this event on the distribution of air pollutants over this state. The model results were evaluated against ERA5 reanalysis, upper air soundings, and TROPOMI-retrieved total column density (TCD) of CO, NO, and O. Two simulations with (Fire) and without (NoFire) biomass burning emissions input were performed to quantify the contribution of forest fires to the concentration of trace gases and particulates. The CO, NO, and O emitted/produced from forest fire over Uttarakhand during April 2022 contributed approximately 39.95, 35.73, and 9.97% to the surface concentration of respective gas. In the case of aerosols, it was around 71.20, 71.44, and 33.62% for PM, PM, and BC respectively. The vertical profile analysis of pollutants revealed that extreme forest fire events can perturb the distribution of air pollutants from the surface up to 450 hPa.