AI Article Synopsis
- The review highlights recent advancements in brightly-emitting materials with different dimensions (0D, 2D, 3D) created using eco-friendly chemistry that exhibit excellent photoluminescence due to self-trapped exciton states.
- It covers 0D emitters like ternary indium-based quantum dots, moves to 2D materials such as single-layer polyheptazine carbon nitride, and discusses 3D luminophores, specifically lead-free double halide perovskites.
- The review concludes with insights on the common characteristics of these materials' photoluminescence and outlines the challenges and future research directions in the area of self-trapped exciton photoluminescence.
Article Abstract
The review summarizes our recent reports on brightly-emitting materials with varied dimensionality (3D, 2D, 0D) synthesized using "green" chemistry and exhibiting highly efficient photoluminescence (PL) originating from self-trapped exciton (STE) states. The discussion starts with 0D emitters, in particular, ternary indium-based colloidal quantum dots, continues with 2D materials, focusing on single-layer polyheptazine carbon nitride, and further evolves to 3D luminophores, the latter exemplified by lead-free double halide perovskites. The review shows the broadband STE PL to be an inherent feature of many materials produced in mild conditions by "green" chemistry, outlining PL features general for these STE emitters and differences in their photophysical properties. The review is concluded with an outlook on the challenges in the field of STE PL emission and the most promising venues for future research.
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| http://dx.doi.org/10.1002/tcr.202300241 | DOI Listing |
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