A method for absolute measurements of the Ac activity in equilibrium with its progeny was developed. Measurements were performed using the triple-to-double coincidence ratio (TDCR) method in two different TDCR counters. The activity concentration of an Ac solution was determined and the solution was sent to the SIR system for a comparison. The half-life of Ac was determined by one of the TDCR counters and found to be 9.9150(63) days.
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http://dx.doi.org/10.1016/j.apradiso.2023.110987 | DOI Listing |
Appl Radiat Isot
December 2024
Radiation Physics Division, National Institute of Standards and Technology, 100 Bureau Dr., Gaithersburg, MD, 20899-8462, USA.
The massic activity of Ac in 0.1 mol/L HCl was measured by multiple primary methods over four consistent measurement campaigns. Results from the triple-to-double coincidence ratio (TDCR) method of liquid scintillation (LS) counting were in accord with other LS-based primary methods.
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December 2024
Bureau International des Poids et Mesures (BIPM), Pavillon de Breteuil, F-92312, Sèvres Cedex, France.
The TDCR (Triple-to-Double Coincidence Ratio) measurement technique is a primary standardization method used by metrology laboratories to accurately determine the activity of radioactive solutions, particularly for radionuclides unsuitable for traditional coincidence counting methods, such as pure beta emitters. The TDCR method leverages a liquid scintillation counter equipped with three photomultiplier tubes (PMTs). This paper introduces TDCRPy, a novel Python package developed by the BIPM, designed to calculate detection efficiency of liquid scintillation counters using Monte Carlo simulations and decay data evaluations from the Decay Data Evaluation Project (DDEP).
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August 2024
Physikalisch-Technische Bundesanstalt (PTB), Bundesallee 100, 38116, Braunschweig, Germany.
A liquid scintillation background sample was measured daily in a custom-built TDCR counter for more than 17 months. The double and triple coincidence counting rates exhibit an annual sinusoidal fluctuation with a maximum in winter and a minimum in summer. Possible correlations with air temperature, air humidity, radon concentration and secondary cosmic radiation were investigated.
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July 2024
Physical Measurement Laboratory, National Institute of Standards and Technology, Gaithersburg, MD 20899, USA.
Appl Radiat Isot
November 2023
Bureau International des Poids et Mesures, Pavillon de Breteuil, 92312, Sèvres, Cedex, France.
A method for absolute measurements of the Ac activity in equilibrium with its progeny was developed. Measurements were performed using the triple-to-double coincidence ratio (TDCR) method in two different TDCR counters. The activity concentration of an Ac solution was determined and the solution was sent to the SIR system for a comparison.
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