A high-brightness ultrabroadband supercontinuum white laser is desirable for various fields of modern science. Here, we present an intense ultraviolet-visible-infrared full-spectrum femtosecond laser source (with 300-5000 nm 25 dB bandwidth) with 0.54 mJ per pulse. The laser is obtained by sending a 3.9 μm, 3.3 mJ mid-infrared pump pulse into a cascaded architecture of gas-filled hollow-core fiber, a bare lithium niobate crystal plate, and a specially designed chirped periodically poled lithium niobate crystal, under the synergic action of second and third order nonlinearities such as high harmonic generation and self-phase modulation. This full-spectrum femtosecond laser source can provide a revolutionary tool for optical spectroscopy and find potential applications in physics, chemistry, biology, material science, industrial processing, and environment monitoring.
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http://dx.doi.org/10.1038/s41377-023-01256-6 | DOI Listing |
Light Sci Appl
August 2023
School of Physics and Optoelectronics, South China University of Technology, Guangzhou, 510641, China.
A high-brightness ultrabroadband supercontinuum white laser is desirable for various fields of modern science. Here, we present an intense ultraviolet-visible-infrared full-spectrum femtosecond laser source (with 300-5000 nm 25 dB bandwidth) with 0.54 mJ per pulse.
View Article and Find Full Text PDFSpectrochim Acta A Mol Biomol Spectrosc
April 2023
College of Optical and Electronic Technology, China Jiliang University, Hangzhou 310018, China. Electronic address:
The in vivo detection of biomarkers in a liquid environment is very important for the early diagnosis of diseases. Spectroscopy methods are employed in ultraviolet-visible-infrared wavelengths, fluorescence or Raman spectra are detected for clinical diagnose. The dual-mode image can provide more diagnostic information and has been realized in some research work.
View Article and Find Full Text PDFResearch (Wash D C)
June 2022
School of Physics and Optoelectronics, South China University of Technology, Guangzhou 510641, China.
Intense ultrabroadband laser source of high pulse energy has attracted more and more attention in physics, chemistry, biology, material science, and other disciplines. We report design and realization of a chirped periodically poled lithium niobate nonlinear crystal that supports ultrabroadband second-harmonic generation covering 350-850 nm by implementing simultaneously up to 12 orders of quasiphase matching against ultrabroadband pump laser covering 700-1700 nm with an average high conversion efficiency of about 25.8%.
View Article and Find Full Text PDFResearch (Wash D C)
March 2021
School of Physics and Optoelectronics, South China University of Technology, Guangzhou 510641, China.
White laser with balanced performance of broad bandwidth, high average and peak power, large pulse energy, high spatial and temporal coherence, controllable spectrum profile, and overall chroma are highly desirable in various fields of modern science. Here, for the first time, we report an innovative scheme of harnessing the synergic action of both the second-order nonlinearity (2-NL) and the third-order nonlinearity (3-NL) in a single chirped periodically poled lithium niobate (CPPLN) nonlinear photonic crystal driven by a high-peak-power near-infrared (NIR) (central wavelength~1400 nm, energy~100 J per pulse) femtosecond pump laser to produce visible to near infrared (vis-NIR, 400-900 nm) supercontinuum white laser. The CPPLN involves a series of reciprocal-lattice bands that can be exploited to support quasiphase matching for simultaneous broadband second- and third-harmonic generations (SHG and THG) with considerable conversion efficiency.
View Article and Find Full Text PDFACS Appl Mater Interfaces
October 2020
School of Physics and Optoelectronic Engineering, Foshan University, Foshan 528000, China.
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