Excitons (coupled electron-hole pairs) in semiconductors can form collective states that sometimes exhibit spectacular nonlinear properties. Here, we show experimental evidence of a collective state of short-lived excitons in a direct-bandgap, atomically thin MoS semiconductor whose propagation resembles that of a classical liquid as suggested by the nearly uniform photoluminescence through the MoS monolayer regardless of crystallographic defects and geometric constraints. The exciton fluid flows over ultralong distances (at least 60 μm) at a speed of ~1.8 × 10 m s (~6% the speed of light). The collective phase emerges above a critical laser power, in the absence of free charges and below a critical temperature (usually T ≈ 150 K) approaching room temperature in hexagonal-boron-nitride-encapsulated devices. Our theoretical simulations suggest that momentum is conserved and local equilibrium is achieved among excitons; both these features are compatible with a fluid dynamics description of the exciton transport.

Download full-text PDF

Source
http://dx.doi.org/10.1038/s41565-023-01438-8DOI Listing

Publication Analysis

Top Keywords

exciton fluid
8
atomically thin
8
thin mos
8
mos semiconductor
8
ultrafast exciton
4
fluid flow
4
flow atomically
4
semiconductor excitons
4
excitons coupled
4
coupled electron-hole
4

Similar Publications

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!