Spatial and spectral characteristics in realizations of broadband terahertz spectroscopy on a subwavelength scale.

In this work, we take aim at the fundamental challenge for realizations of broadband terahertz (THz) spectroscopy on a subwavelength scale. We introduce apertured THz microjets in this effort to resolve the fundamental limits of spatial resolution and spectral bandwidth. The THz microjets are formed as intense foci at the rear of engineered (microcomposite) spheres and are coupled through subwavelength (circular) apertures. Such coupling enables effective transmission of THz power through samples with broad spectral bandwidths and fine spatial resolutions. We show that the apertures function as high-pass filters, with their diameter d enabling strong transmission above a cutoff frequency f. Our theoretical and experimental results reveal that the values for d and f are prescribed by a fixed spatial-spectral product df, whereby reductions in d (to improve the spatial resolution) can raise f into the targeted spectrum (at the expense of spectral bandwidth). We use this understanding to demonstrate broadband (0.3-0.7 THz) THz spectroscopy of lactose at the subwavelength (365 µm) scale. These results for apertured THz microjets represent a 20-fold improvement in spatial resolution over analogous apertured THz plane waves. Overall, our findings show promise for studies of carcinogenesis, pathogenesis, and the like.