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Reductive Fractionation of Flax Shives in Ethanol Medium over RuNi Bimetallic Catalysts. | LitMetric

Reductive Fractionation of Flax Shives in Ethanol Medium over RuNi Bimetallic Catalysts.

Int J Mol Sci

Institute of Chemistry and Chemical Technology, Krasnoyarsk Science Center, Siberian Branch, Russian Academy of Sciences, Akademgorodok 50, Bld. 24, 660036 Krasnoyarsk, Russia.

Published: July 2023

AI Article Synopsis

Article Abstract

The reductive catalytic fractionation of flax shives in the presence of bimetallic NiRu catalysts supported on oxidized carbon materials (CM) such as mesoporous Sibunit and carbon mesostructured by KAIST (CMK-3) was studied. The catalysts based on CMK-3 were characterized by a higher surface area (1216 m/g) compared to the ones based on Sibunit (315 m/g). The catalyst supported on CMK-3 (10Ni3RuC400) was characterized by a more uniform distribution of Ni particles, in contrast to the Sibunit-based catalyst (10Ni3RuS450), on the surface of which large agglomerated particles (300-400 nm) were presented. The bimetallic catalysts were found to be more selective towards propanol-substituted methoxyphenols compared to monometallic Ru/C and Ni/C catalysts. A high yield of monomers (up to 26 wt%, including 17% 4-propanol guaiacol) was obtained in the presence of a 10Ni3RuC400 catalyst based on CMK-3.

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Source
http://www.ncbi.nlm.nih.gov/pmc/articles/PMC10380090PMC
http://dx.doi.org/10.3390/ijms241411337DOI Listing

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