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Precise Synthesis of 4.75 V-Tolerant LiCoO with Homogeneous Delithiation and Reduced Internal Strain.
J Am Chem Soc
January 2025
College of Engineering and Applied Sciences, Jiangsu Key Laboratory of Artificial Functional Materials, National Laboratory of Solid State Microstructures, Collaborative Innovation Centre of Advanced Microstructures, Nanjing University, Nanjing 210093, P. R. China.
The rapid advancements in 3C electronic devices necessitate an increase in the charge cutoff voltage of LiCoO to unlock a higher energy density that surpasses the currently available levels. However, the structural devastation and electrochemical decay of LiCoO are significantly exacerbated, particularly at ≥4.5 V, due to the stress concentration caused by more severe lattice expansion and shrinkage, coupled with heterogeneous Li intercalation/deintercalation reactions.
View Article and Find Full Text PDFDebonding Characteristic and Survival Probability of Adhesive Flash-Free Ceramic Orthodontic Brackets Following pH Cycling.
Eur J Dent
December 2024
Department of Dental Biomaterials, Faculty of Dentistry, Mansoura University, Mansoura City, Egypt.
Objectives: Orthodontic bracket bond failure is an obstacle in clinical orthodontics. This study investigated the influence of pH cycling on the shear bond strength (SBS), adhesive remnant index (ARI), and survival probability of adhesive-precoated flash-free ceramic brackets.
Materials And Methods: Forty mandibular premolars were randomly divided into two groups ( = 20): C: noncoated orthodontic brackets, and F: flash-free adhesive-precoated orthodontic brackets.
Ultra-Flexible High-Linearity Silicon Nanomembrane Synaptic Transistor Array.
Adv Mater
January 2025
School of Electronic and Computer Engineering, Peking University, Shenzhen, 518055, China.
The increasing demand for mobile artificial intelligence applications has elevated edge computing to a prominent research area. Silicon materials, renowned for their excellent electrical properties, are extensively utilized in traditional electronic devices. However, the development of silicon materials for flexible neuromorphic computing devices encounters great challenges.
View Article and Find Full Text PDFUltra robust negative differential resistance memristor for hardware neuron circuit implementation.
Nat Commun
January 2025
Key Laboratory of Brain like Neuromorphic Devices and Systems of Hebei Province, College of Physics Science and Technology, Hebei University, Baoding, Hebei, China.
Neuromorphic computing holds immense promise for developing highly efficient computational approaches. Memristor-based artificial neurons, known for due to their straightforward structure, high energy efficiency, and superior scalability, which enable them to successfully mimic biological neurons with electrical devices. However, the reliability of memristors has always been a major obstacle in neuromorphic computing.
View Article and Find Full Text PDFEngineering synthetic phosphorylation signaling networks in human cells.
Science
January 2025
Department of Bioengineering, Rice University, Houston, TX, USA.
Protein phosphorylation signaling networks have a central role in how cells sense and respond to their environment. We engineered artificial phosphorylation networks in which reversible enzymatic phosphorylation cycles were assembled from modular protein domain parts and wired together to create synthetic phosphorylation circuits in human cells. Our design scheme enabled model-guided tuning of circuit function and the ability to make diverse network connections; synthetic phosphorylation circuits can be coupled to upstream cell surface receptors to enable fast-timescale sensing of extracellular ligands, and downstream connections can regulate gene expression.
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