As renewable electricity becomes cost competitive with fossil fuel energy sources and environmental concerns increase, the transition to electrified chemical and fuel synthesis pathways becomes increasingly desirable. However, electrochemical systems have traditionally taken many decades to reach commercial scales. Difficulty in scaling up electrochemical synthesis processes comes primarily from difficulty in decoupling and controlling simultaneously the effects of intrinsic kinetics and charge, heat, and mass transport within electrochemical reactors. Tackling this issue efficiently requires a shift in research from an approach based on small datasets, to one where digitalization enables rapid collection and interpretation of large, well-parameterized datasets, using artificial intelligence (AI) and multi-scale modeling. In this perspective, we present an emerging research approach that is inspired by smart manufacturing (SM), to accelerate research, development, and scale-up of electrified chemical manufacturing processes. The value of this approach is demonstrated by its application toward the development of CO electrolyzers.
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http://dx.doi.org/10.1016/j.isci.2023.106966 | DOI Listing |
Water Res
December 2024
Department of Global Smart City, Sungkyunkwan University (SKKU), 2066, Seobu-ro, Jangan-gu, Suwon, Gyeonggi-do, 16419, Republic of Korea. Electronic address:
Talanta
December 2024
University of Lodz, Department of Inorganic and Analytical Chemistry, Electroanalysis and Electrochemistry Group, Faculty of Chemistry, Tamka 12, 91-403, Lodz, Poland. Electronic address:
This article describes the effect of non-stabilized magnetic particles FeO (nanoparticles aggregates) addition to the aqueous phase of the polarized liquid-liquid interface (LLI) on the interfacial ion transfer processes. LLI was formed between 1,2-dichloroethane and water solutions (1,2 DCE)|water. The synthesis of FeO magnetic particles (MPs) was achieved by the co-precipitation method, after which their appearance, size of aggregates, and zeta potential were assessed.
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December 2024
Institute of Chemistry and Processes for Energy, Environment and Health (ICPEES), ECPM, UMR 7515 CNRS-University of Strasbourg, 25 rue Becquerel, 67087, Strasbourg, Cedex 02, France.
The increasing availability of electrical energy generated from clean, low-carbon, renewable sources like solar and wind power is paving the way for a more sustainable future. This has resulted in a growing trend in the chemical industry to increase the share of electricity use in chemical processes, particularly catalytic ones. This shift towards electrifying catalytic processes offers significant environmental benefits.
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December 2024
School of Chemical and Biomolecular Engineering, Georgia Institute of Technology, Atlanta, Georgia 30309, United States.
Efforts addressing sludge management, food security, and resource recovery have led to novel approaches in these areas. Electrically assisted conversion of sludge stands out as a promising technology for sewage sludge valorization, producing nitrogen and phosphorus-based fertilizers. The adoption of this technology, which could lead to a fertilizer circular economy, holds the potential to catalyze a transformative change in wastewater treatment facilities toward process intensification, innovation, and sustainability.
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December 2024
Department of Chemical Engineering, National Taiwan University of Science and Technology, Taipei, 10607, Taiwan.
Controlling the redox ability is crucial for optimizing catalytic processes in clean energy, environmental protection, and CO reduction, as it directly influences the reaction efficiency and electron transfer rates, driving sustainable and effective outcomes. Here, we report the plasma-electrified synthesis of composition-controlled FeAu bimetallic nanoparticles, specifically engineered to enhance the redox catalytic performance through precise tuning of their chemical states. Utilizing atmospheric-pressure microplasmas, FeAu nanoparticles were synthesized under ambient conditions without the need for reducing agents or organic solvents, thereby providing a green and sustainable approach.
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