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Applications of Verdazyl Radicals in Energy Storage, Molecular Electronics and Magnetism: Teaching Old Molecules New Tricks.
Chem Asian J
January 2025
University of Tasmania, School of Natural Sciences - Chemistry, AUSTRALIA.
Verdazyls are a fundamental class of stable organic radicals that have been traditionally overshadowed by the more synthetically accessible stable nitroxide radicals. With the advent of enhanced synthetic routes to verdazyls, particularly in recent years, these systems are now poised to realise their potential in a range of applications across emerging technologies that will be important to addressing challenges faced by modern society. This Concept discusses the enabling properties of a selection of verdazyl-based systems that feature promising applications in energy storage, molecular electronics and magnetic molecules.
View Article and Find Full Text PDFA focus on microporous perovskites: new tricks for an old dog.
Chem Sci
January 2025
Laboratorio de Fisicoquímica y Reactividad de Superficies (LaFReS), Instituto de Investigaciones en Materiales, Universidad Nacional Autónoma de México Circuito Exterior s/n, CU, Coyoacán 04510 Ciudad de México Mexico
Hybrid organic-inorganic perovskites (HOIPs) are widely studied for their potential in optoelectronic devices due to their unique semiconductor features. Porous HOIPs are extremely rare, with (APOSS)[CuCl] being one of the very few examples, featuring 12 Å pores within its lattice. Reed and coworkers (C.
View Article and Find Full Text PDFOrganocatalytic Hat Trick: 1,5,7-Triazabicyclo[4.4.0]dec-5-ene (TBD)-Catalyzed Synthesis of Cyclic Imides via an Amidation-Cyclization-Elimination Cascade.
J Org Chem
January 2025
Department of Chemistry, McGill University, 801 Sherbrooke Street West, Montreal, Quebec H3A 0B8, Canada.
1,5,7-Triazabicyclo[4.4.0]dec-5-ene (TBD) was used for the synthesis of cyclic imides via an amidation-cyclization-elimination cascade.
View Article and Find Full Text PDFDeterminism of formamide-based biogenic prebiotic reactions.
Phys Life Rev
December 2024
Department of Ecological and Biological Sciences, Via San Camillo De Lellis, Università della Tuscia, Viterbo 01100, Italy. Electronic address:
Article Synopsis
- Formamide, when reacting with a catalyst and energy, produces a variety of important compounds like amino acids, sugars, and nucleic bases, which are the building blocks of life.
- Different catalysts yield unique product sets, but there's significant overlap in the types of compounds formed, indicating a robust chemical process.
- The findings suggest that the early conditions on Earth for creating life-like molecules were straightforward and did not require unusual environments, supporting the idea of a predictable prebiotic chemistry.
Article Synopsis
- The Sir2 enzyme (Sir2A) is crucial for the antigenic variation of malaria parasites, and inhibiting it could lead to new treatments.
- Current challenges in finding selective inhibitors stem from Sir2A's weak deacetylase activity, but this study characterizes its activity and uncovers potential inhibitors.
- The research finds that Sir2A is more active with nucleosome substrates and identifies myristic acid as a regulator, leading to the discovery of synthetic small molecule inhibitors that could aid in developing antimalarial therapies.
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