The shortage of drinking water has become a global problem, coastal cities can make full use of abundant seawater resources by desalination technology to ease the contradiction between supply and demand. However, fossil energy consumption contradicts the goal of reducing carbon dioxide emissions. Currently, researchers favor interfacial solar desalination devices relying only on clean solar energy. Based on the structure optimization of the evaporator, a kind of device composed of a superhydrophobic BiOI (BiOI-FD) floating layer and CuO polyurethane sponge (CuO sponge) is constructed in this paper, with its design advantages presented in the following two aspects: 1. The novel BiOI-FD photocatalyst in the floating layer reduces the surface tension and realizes the degradation of the enriched pollutants, ensuring the device to achieve solar desalination and inland sewage purification; 2. CuO sponge can inhibit salt crystallization and realize the combination of the water transport and photothermal layers. Particularly, the photothermal evaporation rate of the interface device reached 2.37 kg m h.The novel interface evaporator design will bring a new solution for solar desalination, sewage treatment and large-scale application.
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http://dx.doi.org/10.1016/j.jcis.2023.06.071 | DOI Listing |
Langmuir
December 2024
Department of Physical Chemistry, Faculty of Chemistry and Petroleum Sciences, Bu-Ali Sina University, Hamedan 65167 ,Iran.
Interfacial solar evaporator generation (ISVG) is a new, cost-effective, and eco-friendly emerging method for water desalination. Two main criteria for evaluating ISVG performance are evaporation rate () and solar-to-vapor conversion efficiency (η). The main challenge of the previously presented models for the estimation of and η in 2D systems is that in most cases the calculated values are beyond the theoretical limits, > 1.
View Article and Find Full Text PDFSci Rep
December 2024
Centre Énergie, Matériaux Télécommunications, Institut National de la Recherche Scientifique, 1650, Blvd, Lionel-Boulet, Varennes, QC, J3X-1P7, Canada.
RF-sputtering is used to deposit TiO-Magneli-phase films onto various substrates at deposition temperatures (T) ranging from 25 to 650 °C. Not only the structural, but also electrical conductivity, optical absorbance and photothermal properties of the TiO films are shown to change significantly with T. A T of 500 °C is pointed out as the optimal temperature that yields highly-crystalized pure-TiO-Magneli phase with a densely-packed morphology and a conductivity as high as 740 S/cm.
View Article and Find Full Text PDFAdv Sci (Weinh)
December 2024
Institute for Frontier Materials, Deakin University, Geelong, VIC, 3216, Australia.
Interfacial solar steam generation (ISSG) employed for seawater desalination and wastewater purification shows great promise to alleviate global freshwater scarcity. However, simultaneous optimization of water transfer direction in a cost-effective and reliable ISSG to balance thermal localization, salt accumulation, and resistance to oilfouling represents a rare feat. Herein, inspired by seabird beaks for unidirectional water transfer, eco-friendly and cost-effective plant extracts, sodium alginate, and tannic acid, are selected for crafting an innovative Sodium Alginate-Tannic Acid Hemispheric Evaporator (STHE).
View Article and Find Full Text PDFAngew Chem Int Ed Engl
December 2024
Luoyang Normal University, College of Chemistry and Chemical Engineering, CHINA.
The synthesis of high-ordered mechanically interlocked supramolecular structures is an extremely challenging topic. Only two linear [4]catenanes have been reported so far and there is no defined strategy to obtain cyclic [4]catenane. Herein, two unprecedented cyclic [4]catenanes, 1 and 2, were prepared in high yields.
View Article and Find Full Text PDFAdv Colloid Interface Sci
December 2024
School of Materials Science and Engineering, Shaanxi Key Laboratory of Green Preparation and Functionalization for Inorganic Materials, Shaanxi University of Science and Technology, Xi'an, Shaanxi 710021, China.
Photothermal conversion materials (PCMs) are crucial component in solar-thermal energy technologies. Although various PCMs with excellent sunlight harvesting have been developed for colorful solar-thermal applications, uniform and large-scale production of PCMs remains a challenge, and the PCMs prepared through the conventional methods are often non-site specific. Laser processing technology (LPT), as an efficient, convenient, green and sustainable technology, can directly create micro/nano structures and patterns at specific locations on materials surface, attracting widespread attention in photo-to-thermal applications.
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