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Controlling the J- and H-Aggregates and Supramolecular Polymerization Pathways of Anthanthrene by Tuning the Hydrogen Bonding Sites.
Chemistry
January 2025
Shaanxi Normal University, School of Chemistry and Chemical Engineering, Shaanxi Normal University, 710119, Xi'an, CHINA.
Exploration of new π-conjugated building blocks for construction of supramolecular polymers is at the forefront of self-assembly. Herein, we incorporate a highly planar anthanthrene skeleton into the design of two supramolecular monomers 1 and 2. Their supramolecular polymerization have been comprehensively investigated by spectroscopic studies.
View Article and Find Full Text PDFRecent progress of mechanofluorochromism and mechanoluminescence for phenothiazine derivatives and analogues.
Chemistry
January 2025
Qinghai University, College of Chemistry, CHINA.
Mechanofluorochromism (MFC) and mechanoluminescence (ML) materials have garnered significant attention from researchers due to their potential applications in anti-counterfeiting, optical recording, photodynamic therapy, bioimaging, stress sensing, display technology, and ink-free printing paper. Among the various building blocks utilized in these materials, phenothiazine (PTZ) has emerged as a widely employed fundamental component owing to its distinctive electronic and optical properties as well as its facile modification capabilities. Summarizing the recent progress of PTZ derivatives and analogues in this field holds practical significance.
View Article and Find Full Text PDFNonlinear Optical Properties of Bis(dehydrobenzoannuleno)benzenes: An Experimental and Computational Approach.
J Phys Chem A
January 2025
Department of Chemistry, University of Michigan, Ann Arbor, Michigan 48109, United States.
Given their molecular properties and electronic structure, graphyne and graphdiyne are promising materials with numerous applications in different fields of material science. Dehydrobenzoannules (DBAs) are candidates that can serve as building blocks for synthesizing and designing new 2D carbon allotropes; however, only a few graphynes have been produced on a practical scale. Herein, we present our investigation of three DBAs, which serve as a model to understand the relationship between the structure and property, contributing to 2D carbon allotropes' rational design and synthetic effort.
View Article and Find Full Text PDFPersistence of the Immune Response to an Intramuscular Bivalent (GI.1/GII.4) Norovirus Vaccine in Adults.
Vaccines (Basel)
January 2025
Clinical Development, Takeda Pharmaceuticals International AG, Farman Strasse 11, Opfikon, 8152 Zurich, Switzerland.
Background: Major global economic and health burdens due to norovirus gastroenteritis could be addressed by an effective vaccine.
Methods: In this study, 428 adult recipients of various compositions of the norovirus vaccine candidate, HIL-214, were followed for 5 years, to assess immune responses to its virus-like particle antigens, GI.1 and GII.
Development of a Cationic Polymeric Micellar Structure with Endosomal Escape Capability Enables Enhanced Intramuscular Transfection of mRNA-LNPs.
Vaccines (Basel)
December 2024
Shenzhen Neocurna Biotechnology Corporation, 12/F, Block B, Building 1, Yinxingzhijie Phase II, Longhua District, Shenzhen 518100, China.
The endosomal escape of lipid nanoparticles (LNPs) is crucial for efficient mRNA-based therapeutics. Here, we present a cationic polymeric micelle (cPM) as a safe and potent co-delivery system with enhanced endosomal escape capabilities. We synthesized a cationic and ampholytic di-block copolymer, poly (poly (ethylene glycol) methacrylate--hexyl methacrylate)--poly(butyl methacrylate--dimethylaminoethyl methacrylate--propyl acrylate) (p(PEGMA--HMA)--p(BMA--DMAEMA--PAA)), via reversible addition-fragmentation chain transfer polymerization.
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