Lead sulfide colloidal quantum dots (PbS CQDs) are promising optoelectronic materials due to their unique properties, such as tunable band gap and strong absorption, which are of immense interest for application in photodetectors and solar cells. However, the tunable band gap of PbS CQDs would only cover visible short-wave infrared; the ability to detect longer wavelengths, such as mid- and long-wave infrared, is limited because they are restricted by the band gap of the bulk material. In this paper, a novel photodetector based on the synergistic effect of PbS CQDs and bismuth telluride (BiTe) was developed for the detection of a mid-wave infrared band at room temperature. The device demonstrated good performance in the visible-near infrared band (i.e., between 660 and 850 nm) with detectivity of 1.6 × 10 Jones at room temperature. It also exhibited photoelectric response in the mid-wave infrared band (i.e., between 4.6 and 5.1 μm). The facile fabrication process and excellent performance (with a response of up to 5.1 μm) of the hybrid BiTe/PbS CQDS photodetector are highly attractive for many important applications that require high sensitivity and broadband light detection.
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http://dx.doi.org/10.3390/s23094328 | DOI Listing |
J Urban Health
January 2025
Department of Geography, Florida State University, Bellamy Building, Room 323, 113 Collegiate Loop, PO Box 3062190, Tallahassee, FL, 32306-2190, USA.
Understanding when and where heat adversely influences health outcomes is critical for targeting interventions and adaptations. However, few studies have analyzed the role of indoor heat exposures on acute health outcomes. To address this research gap, the study partnered with the New York City Fire Department Emergency Medical Services.
View Article and Find Full Text PDFACS Appl Mater Interfaces
January 2025
School of Artificial Intelligence Science and Technology, University of Shanghai for Science and Technology, Shanghai 200093, China.
Passive radiative cooling has recently gained significant attention as a highly promising technology that offers a zero-energy and electricity-free solution to tackle the pressing issue of global warming. Nevertheless, research efforts have predominantly focused on enhancing daytime and hot-day radiative cooling efficacy, often neglecting the potential downsides associated with excessive cooling and the consequent increased heating expenses during cold nights and winter days. Herein, we demonstrate a micro-nanostructured engineered composite film that synergistically integrates room-temperature adaptive silica-shell/oil-core phase change microcapsules (S-PCMs) with commercially available cellulose fibers.
View Article and Find Full Text PDFACS Appl Mater Interfaces
January 2025
School of Materials Science and Engineering, Shanghai JiaoTong University 800 Dongchuan Road, Shanghai 200240, P. R. China.
Solid polymer electrolytes (SPEs) with excellent ionic conductivity and a wide electrochemical stability window are critical for high-energy lithium metal batteries (LMBs). However, the widespread application of polymer electrolytes is severely limited by inadequate room-temperature ionic conductivity, sluggish interfacial charge transport, and uncontrolled reactions at the electrode/electrolyte interface. Herein, we present a uniform polymerized 1,3-dioxolane (PDOL) composite solid polymer electrolyte (PDOL-S/F-nano LiF CSE) that satisfies these requirements through the in situ catalytic polymerization effect of nano LiF on the polymerization of 1,3-dioxolane-based electrolytes.
View Article and Find Full Text PDFJ Colloid Interface Sci
January 2025
School of Chemical Sciences, University of Chinese Academy of Sciences, Beijing 101408 China. Electronic address:
The exploration of pure organic ultra-long room temperature phosphorescence (RTP) materials has emerged as a research hotspot in recent years. Herein, a simple strategy for fabricating long-afterglow polymer aerogels with three-dimensional ordered structures and environmental monitoring capabilities is proposed. Based on the non-covalent interactions between pectin (PC) and melamine formaldehyde (MF), a composite aerogel (PCMF@phenanthrene) (PCMF@PA) doped with phosphorescent organic small molecules was constructed.
View Article and Find Full Text PDFAppl Radiat Isot
January 2025
Department of Physics, Faculty of Science, Universiti Teknologi Malaysia, 81300, Skudai, Johor, Malaysia.
Dealing with radioactive waste, particularly from various industrial processes, poses significant challenges. This paper explores the use of lithium aluminate borate (Li-Al-B) glass matrix as an alternative method for immobilizing radioactive waste, focusing specifically on waste generated in tin smelting industries, known as tin slag. The study primarily concentrates on transforming tin slag, a byproduct abundant in Natural Occurring Radioactive Material (NORM), into a stable and safe form for disposal.
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