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Janus Metal-Organic Framework Membranes Boosting the Osmotic Energy Harvesting. | LitMetric

Janus Metal-Organic Framework Membranes Boosting the Osmotic Energy Harvesting.

ACS Appl Mater Interfaces

State Key Laboratory of Analytical Chemistry for Life Science, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing 210023, China.

Published: May 2023

AI Article Synopsis

  • * Researchers created a Janus metal-organic framework (J-MOF) membrane using an electrodeposition technique, which allows for quick ion transport and excellent ion selectivity.
  • * The J-MOF's design, with its asymmetric structure, effectively minimizes ion concentration polarization and boosts charge separation, resulting in a notable output power density of 3.44 W/m at a high concentration gradient.

Article Abstract

The unique ion-transport properties in nanoconfined pores enable nanofluidic devices with great potential in harvesting osmotic energy. The energy conversion performance could be significantly improved by the precise regulation of the "permeability-selectivity" trade-off and the ion concentration polarization effect. Here, we take the advantage of electrodeposition technique to fabricate a Janus metal-organic framework (J-MOF) membrane that possesses rapid ion-transport capability and impeccable ion selectivity. The asymmetric structure and asymmetric surface charge distribution of the J-MOF device can suppress the ion concentration polarization effect and enhance the ion charge separation, exhibiting an improved energy harvesting performance. An output power density of 3.44 W/m has been achieved with the J-MOF membrane at a 1000-fold concentration gradient. This work provides a new strategy for fabricating high-performance energy-harvesting devices.

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Source
http://dx.doi.org/10.1021/acsami.3c01936DOI Listing

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