AI Article Synopsis
- The magnetic properties of a single crystal (FeMn)MoO were analyzed, revealing an antiferromagnetic state for lower Mn content (≤ 0.25) and a ferrimagnetic phase for higher Mn content (≥ 0.3).
- All samples displayed significant electric polarization related to spin, regardless of their magnetic state.
- The ferrimagnetic samples showed distinct square-like magnetic hysteresis loops, with changes in remnant magnetization and coercive field linked to variations in Mn content and temperature.
Article Abstract
In the present work, the magnetic properties of a single crystal (FeMn)MoO (0 ≤ ≤ 1) have been studied by performing extensive measurements. A detailed magnetic phase diagram is built up, in which the antiferromagnetic state dominates for ≤ 0.25 and the ferrimagnetic phase arises for ≥ 0.3. Meanwhile, a sizeable electric polarization of spin origin is commonly observed in all samples, no matter what the magnetic state is. For the samples hosting a ferrimagnetic state, square-like magnetic hysteresis loops are revealed, while the remnant magnetization and coercive field can be tuned drastically by simply varying the Mn content or temperature. A possible coexistence of the antiferromagnetic and ferrimagnetic phases is proposed to be responsible for the remarkable modulation of magnetic properties in the samples.
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| http://dx.doi.org/10.1021/acsami.3c00518 | DOI Listing |
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