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Post-synthetic atomically precise single-Cu sites in a thiacalix[4]arene-supported octahedral Na@Co cluster: the Cu-Co synergistic effect for selective photocatalytic conversion of CO to CO. | LitMetric
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Post-synthetic atomically precise single-Cu sites in a thiacalix[4]arene-supported octahedral Na@Co cluster: the Cu-Co synergistic effect for selective photocatalytic conversion of CO to CO.

Yinjuan Guo Jiahui Li Guiyan Zhao Baokuan Chen Xinxin Hang Yanfeng Bi

Chem Commun (Camb)

School of Petrochemical Engineering, Liaoning Petrochemical University, Fushun, Liaoning 113001, P. R. China.

Published: May 2023

A thiacalix[4]arene-supported octahedral Na@Co cluster has been fabricated by the modular assembly of six Co-(TC4A) polynuclear secondary building units (PSBUs) and eight 2,4,6-PTC linkers. The post-modification of Na@Co by ion exchange of Na with Cu on the surface of the octahedron afforded a structurally well-defined Cu@Co cluster. The obtained Cu@Co cluster achieved improved visible-light absorption and selective photoreduction of CO to CO due to the Cu-Co synergistic effect.

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http://dx.doi.org/10.1039/d3cc01230aDOI Listing

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