Masers can deliver ultralow-noise amplification of microwave signals in medical imaging and deep-space communication, with recent research being rekindled through the discovery of gain media operating at room-temperature, eschewing bulky cryogenics that hindered their use. This work shows the discovery of 6,13-diazapentacene doped in para-terphenyl (DAP:PTP) as a maser gain medium that can operate at room-temperature, without an external magnetic field. With a maser output power of -10 dBm, it is on par with pentacene-doped para-terphenyl in masing power, while possessing compelling advantages such as faster amplification startup times, being pumped by longer wavelength light at 620 nm and greater chemical stability from nitrogen groups. Furthermore, the maser bursts from DAP:PTP allow one to reach the strong coupling regime for cavity quantum electrodynamics, with a high cooperativity of 182. The optical and microwave spin dynamics of DAP:PTP are studied in order to evaluate its capabilities as a maser gain medium, where it features fast intersystem crossing and an advantageously higher triplet quantum yield. The results pave the way for the future discovery of similar maser materials and help designate them as promising candidates for quantum sensors, optoelectronic devices and the study of cavity quantum electrodynamic effects at room-temperature.

Download full-text PDF

Source
http://dx.doi.org/10.1002/adma.202300441DOI Listing

Publication Analysis

Top Keywords

cavity quantum
12
strong coupling
8
quantum electrodynamics
8
maser gain
8
gain medium
8
maser
6
quantum
5
move pentacene
4
pentacene diazapentacene-doped
4
diazapentacene-doped para-terphenyl
4

Similar Publications

Low-threshold surface-emitting colloidal quantum-dot circular Bragg laser array.

Light Sci Appl

January 2025

State Key Laboratory of Optical Fiber and Cable Manufacture Technology, Institute of Nanoscience and Applications, Department of Electrical and Electronic Engineering, Southern University of Science and Technology, Shenzhen, China.

Colloidal quantum dots (CQDs) are attractive gain media due to their wavelength-tunability and low optical gain threshold. Consequently, CQD lasers, especially the surface-emitting ones, are promising candidates for display, sensing and communication. However, it remains challenging to achieve a low-threshold surface-emitting CQD laser array with high stability and integration density.

View Article and Find Full Text PDF

Enhancement of quantum synchronization in triple-cavity system.

Sci Rep

January 2025

School of Physics and Optoelectronics, Xiangtan University, Xiangtan, 411105, China.

We introduce two strategies to enhance quantum synchronization within a triple-cavity optomechanical system, where each cavity contains an oscillator and is interconnected via optical fibers. Our results demonstrate that applying appropriate periodic modulation to the driving fields or the cavity modes can ensure robust quantum synchronization across both open and closed configurations. This approach offers promising avenues for expanding quantum synchronization capabilities in multi-cavity systems and has significant implications for advancing quantum synchronization generation and application in complex networks.

View Article and Find Full Text PDF

Enhanced Light-Matter Interaction with Bloch Surface Wave Modulated Plasmonic Nanocavities.

Nano Lett

January 2025

State Key Laboratory for Mesoscopic Physics and Frontiers Science Center for Nano-optoelectronics, School of Physics, Peking University, 100871 Beijing, China.

Article Synopsis
  • Strong coupling between nanocavities and single excitons at room temperature is crucial for studying cavity quantum electrodynamics, influenced by factors like light confinement and electric field orientation.
  • A hybrid cavity design combining a one-dimensional photonic crystal and plasmonic nanocavity enhances quality factor, minimizes mode volume, and allows control of electric field direction using Bloch surface waves.
  • Achieving a Rabi splitting of around 186 meV with only 8 excitons involved marks a significant advance, producing an effective coupling strength of 17.6 meV per exciton, which is nearly double the previously reported values for TMD-based systems.
View Article and Find Full Text PDF

Interaction-Enhanced Superradiance of a Rydberg-Atom Array.

Phys Rev Lett

December 2024

CAS Key Laboratory of Quantum Information, University of Science and Technology of China, Hefei 230026, China.

We study the superradiant phase transition of an array of Rydberg atoms in a dissipative microwave cavity. Under the interplay of the cavity field and the long-range Rydberg interaction, the steady state of the system exhibits an interaction-enhanced superradiance, with vanishing critical atom-cavity coupling rates at a discrete set of interaction strengths. We find that, while the phenomenon can be analytically understood in the case of a constant all-to-all interaction, the enhanced superradiance persists under typical experimental parameters with spatially dependent interactions, but at modified critical interaction strengths.

View Article and Find Full Text PDF

Reinforcement Learning Optimization of the Charging of a Dicke Quantum Battery.

Phys Rev Lett

December 2024

Freie Universität Berlin, Department of Mathematics and Computer Science, Arnimallee 6, 14195 Berlin, Germany.

Quantum batteries are energy-storing devices, governed by quantum mechanics, that promise high charging performance thanks to collective effects. Because of its experimental feasibility, the Dicke battery-which comprises N two-level systems coupled to a common photon mode-is one of the most promising designs for quantum batteries. However, the chaotic nature of the model severely hinders the extractable energy (ergotropy).

View Article and Find Full Text PDF

Want AI Summaries of new PubMed Abstracts delivered to your In-box?

Enter search terms and have AI summaries delivered each week - change queries or unsubscribe any time!