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Dynamical susceptibilities near ideal glass transitions. | LitMetric

Dynamical susceptibilities near ideal glass transitions.

Phys Rev E

Soft Matter & Biological Physics, Department of Applied Physics, Eindhoven University of Technology, P.O. Box 513, 5600MB Eindhoven, The Netherlands.

Published: December 2022

Building on the recently derived inhomogeneous mode-coupling theory, we extend the generalized mode-coupling theory of supercooled liquids to inhomogeneous environments. This provides a first-principles-based, systematic, and rigorous way of deriving high-point dynamical susceptibilities from variations of the many-body dynamic structure factors with respect to their conjugate field. This framework allows for a fully microscopic possibility to probe for collective relaxation mechanisms in supercooled liquids near the mode-coupling glass transition. The behavior of these dynamical susceptibilities is then studied in the context of simplified self-consistent relaxation models.

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http://dx.doi.org/10.1103/PhysRevE.106.064136DOI Listing

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