We report a H evolving hybrid photocathode based on SbSe and a precious metal free molecular catalyst. Through the use of a high surface area TiO scaffold, we successfully increased the Ni molecular catalyst loading from 7.08 ± 0.43 to 45.76 ± 0.81 nmol cm, achieving photocurrents of 1.3 mA cm at 0 V RHE, which is 81-fold higher than the device without the TiO mesoporous layer.
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| http://dx.doi.org/10.1039/d2cc04810h | DOI Listing |
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