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Controllable multi-halogenation of a non-native substrate by SyrB2 iron halogenase.
bioRxiv
May 2024
Department of Chemistry, University of Minnesota, Twin Cities, Minneapolis, MN, 55455, United States.
Geminal, multi-halogenated functional groups are widespread in natural products and pharmaceuticals, yet no synthetic methodologies exist that enable selective multi-halogenation of unactivated C-H bonds. Biocatalysts are powerful tools for late-stage C-H functionalization, as they operate with high degrees of regio-, chemo-, and stereoselectivity. 2-oxoglutarate (2OG)-dependent non-heme iron halogenases chlorinate and brominate aliphatic C-H bonds offering a solution for achieving these challenging transformations.
View Article and Find Full Text PDFA multihalogenation strategy for ambipolar transistors and high-gain inverters with good noise margin.
Sci Bull (Beijing)
September 2022
Beijing National Laboratory for Molecular Sciences, Key Laboratory of Organic Solids, Institute of Chemistry Chinese Academy of Sciences, Beijing 100190, China. Electronic address:
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